DOI: 10.1557/mrs2007.208. Novel<i>In Situ</i>Probes for Nanocatalysis

10.1557/mrs2007.208

Crossref journal-article

Springer Science and Business Media LLC

MRS Bulletin (297)

Abstract

AbstractDuring the past few years, substantial effort has been devoted to developing new experimental techniques capable of delivering atomic-scale information on surfaces and nanoparticles under catalytic reaction conditions. Since the advent of surface science, pioneering experiments under highly idealized conditions have been performed (at very low gas pressures, <10−6mbar), and idealized model material systems (e.g., single crystals) have been investigated. However, understanding chemical reactions on singlecrystal surfaces close to ultrahigh vacuum does not always enable prediction of the performance of nanoparticles operating at gas pressures near or above atmospheric pressure. Therefore, thisMRS Bulletinissue focuses on the capabilities of atomic-scaleresolution, high-gas-pressure- and high-temperature-compatiblein situprobes sensitive to the structure, chemical composition, and dynamical properties of nanomaterials. It will be demonstrated how novelin situtechniques enable one to bridge the combined pressure and materials gaps from ultrahigh vacuum to atmospheric pressures and from metal single-crystal surfaces to nanoparticles or oxides.

Bibliography

Stierle, A., & Molenbroek, A. M. (2007). NovelIn SituProbes for Nanocatalysis. MRS Bulletin, 32(12), 1001â1009.

Authors 2

Andreas Stierle (first)
Alfons M. Molenbroek (additional)

References 31 Referenced 51

10.1038/nature02278
10.1063/1.1824351
10.1103/PhysRevLett.86.460
10.1016/S0360-0564(02)45018-3 / Adv. Catal. by McCrea (2000)
10.1557/mrs2006.175
10.1023/A:1016686322301
10.1063/1.1389497
10.1021/jp0715631
10.1103/PhysRevLett.98.046101
{'key': 'S0883769400008721_ref001', 'volume-title': 'Handbook of Heterogeneous Catalysis', 'author': 'G.', 'year': '1997'} / Handbook of Heterogeneous Catalysis by G. (1997)
10.1039/b100115a
10.1016/S0167-5729(98)00002-8
10.1002/9783527611348
10.1016/0921-4526(94)00655-F
10.1103/PhysRevLett.86.5325
10.1063/1.1841951
10.1021/ja055754y
10.1103/PhysRevLett.85.776
10.1016/j.susc.2004.01.025
10.1116/1.578531
10.1103/PhysRevB.61.213
10.1103/PhysRevLett.95.255505
10.1080/01614949208021918 / Cat. Rev. Sci. Eng. by Gai (1992)
10.1016/j.ultramic.2006.01.006
10.1016/j.surfrep.2005.03.002
10.1126/science.1082146
10.1016/S1381-1169(97)00270-7
10.1016/j.susc.2006.05.030
10.1016/S0360-0564(06)51004-1 / Adv. Catal. by Rupprechter (2007)
10.1039/b504027b
10.1016/0920-5861(91)85023-2

Dates

Type	When
Created	14 years, 6 months ago (Feb. 2, 2011, 7:42 a.m.)
Deposited	1 year, 4 months ago (April 3, 2024, 3:21 p.m.)
Indexed	2 months, 2 weeks ago (June 16, 2025, 6:44 p.m.)
Issued	17 years, 8 months ago (Dec. 1, 2007)
Published	17 years, 8 months ago (Dec. 1, 2007)
Published Online	14 years, 7 months ago (Jan. 31, 2011)
Published Print	17 years, 8 months ago (Dec. 1, 2007)

Funders 0

None

BibTeX

@article{Stierle_2007, title={NovelIn SituProbes for Nanocatalysis}, volume={32}, ISSN={1938-1425}, url={http://dx.doi.org/10.1557/mrs2007.208}, DOI={10.1557/mrs2007.208}, number={12}, journal={MRS Bulletin}, publisher={Springer Science and Business Media LLC}, author={Stierle, Andreas and Molenbroek, Alfons M.}, year={2007}, month=dec, pages={1001–1009} }

JSON

{
  "indexed": {
    "date-parts": [
      [
        2025,
        6,
        16
      ]
    ],
    "date-time": "2025-06-16T22:44:58Z",
    "timestamp": 1750113898941
  },
  "reference-count": 31,
  "publisher": "Springer Science and Business Media LLC",
  "issue": "12",
  "license": [
    {
      "start": {
        "date-parts": [
          [
            2011,
            1,
            31
          ]
        ],
        "date-time": "2011-01-31T00:00:00Z",
        "timestamp": 1296432000000
      },
      "content-version": "unspecified",
      "delay-in-days": 1157,
      "URL": "https://www.cambridge.org/core/terms"
    }
  ],
  "content-domain": {
    "domain": [],
    "crossmark-restriction": false
  },
  "published-print": {
    "date-parts": [
      [
        2007,
        12
      ]
    ]
  },
  "abstract": "<jats:title>Abstract</jats:title><jats:p>During the past few years, substantial effort has been devoted to developing new experimental techniques capable of delivering atomic-scale information on surfaces and nanoparticles under catalytic reaction conditions. Since the advent of surface science, pioneering experiments under highly idealized conditions have been performed (at very low gas pressures, &lt;10<jats:sup>\u22126</jats:sup>mbar), and idealized model material systems (e.g., single crystals) have been investigated. However, understanding chemical reactions on singlecrystal surfaces close to ultrahigh vacuum does not always enable prediction of the performance of nanoparticles operating at gas pressures near or above atmospheric pressure. Therefore, this<jats:italic>MRS Bulletin</jats:italic>issue focuses on the capabilities of atomic-scaleresolution, high-gas-pressure- and high-temperature-compatible<jats:italic>in situ</jats:italic>probes sensitive to the structure, chemical composition, and dynamical properties of nanomaterials. It will be demonstrated how novel<jats:italic>in situ</jats:italic>techniques enable one to bridge the combined pressure and materials gaps from ultrahigh vacuum to atmospheric pressures and from metal single-crystal surfaces to nanoparticles or oxides.</jats:p>",
  "DOI": "10.1557/mrs2007.208",
  "type": "journal-article",
  "created": {
    "date-parts": [
      [
        2011,
        2,
        2
      ]
    ],
    "date-time": "2011-02-02T12:42:09Z",
    "timestamp": 1296650529000
  },
  "page": "1001-1009",
  "source": "Crossref",
  "is-referenced-by-count": 51,
  "title": "Novel<i>In Situ</i>Probes for Nanocatalysis",
  "prefix": "10.1557",
  "volume": "32",
  "author": [
    {
      "given": "Andreas",
      "family": "Stierle",
      "sequence": "first",
      "affiliation": []
    },
    {
      "given": "Alfons M.",
      "family": "Molenbroek",
      "sequence": "additional",
      "affiliation": []
    }
  ],
  "member": "297",
  "published-online": {
    "date-parts": [
      [
        2011,
        1,
        31
      ]
    ]
  },
  "reference": [
    {
      "key": "S0883769400008721_ref030",
      "doi-asserted-by": "publisher",
      "DOI": "10.1038/nature02278"
    },
    {
      "key": "S0883769400008721_ref020",
      "doi-asserted-by": "publisher",
      "DOI": "10.1063/1.1824351"
    },
    {
      "key": "S0883769400008721_ref004",
      "doi-asserted-by": "publisher",
      "DOI": "10.1103/PhysRevLett.86.460"
    },
    {
      "key": "S0883769400008721_ref021",
      "doi-asserted-by": "crossref",
      "first-page": "385",
      "DOI": "10.1016/S0360-0564(02)45018-3",
      "volume": "45",
      "author": "McCrea",
      "year": "2000",
      "journal-title": "Adv. Catal."
    },
    {
      "key": "S0883769400008721_ref002",
      "doi-asserted-by": "publisher",
      "DOI": "10.1557/mrs2006.175"
    },
    {
      "key": "S0883769400008721_ref007",
      "doi-asserted-by": "publisher",
      "DOI": "10.1023/A:1016686322301"
    },
    {
      "key": "S0883769400008721_ref016",
      "doi-asserted-by": "publisher",
      "DOI": "10.1063/1.1389497"
    },
    {
      "key": "S0883769400008721_ref006",
      "doi-asserted-by": "publisher",
      "DOI": "10.1021/jp0715631"
    },
    {
      "key": "S0883769400008721_ref003",
      "doi-asserted-by": "publisher",
      "DOI": "10.1103/PhysRevLett.98.046101"
    },
    {
      "key": "S0883769400008721_ref001",
      "volume-title": "Handbook of Heterogeneous Catalysis",
      "author": "G.",
      "year": "1997"
    },
    {
      "key": "S0883769400008721_ref026",
      "doi-asserted-by": "publisher",
      "DOI": "10.1039/b100115a"
    },
    {
      "key": "S0883769400008721_ref011",
      "doi-asserted-by": "publisher",
      "DOI": "10.1016/S0167-5729(98)00002-8"
    },
    {
      "key": "S0883769400008721_ref024",
      "doi-asserted-by": "publisher",
      "DOI": "10.1002/9783527611348"
    },
    {
      "key": "S0883769400008721_ref027",
      "doi-asserted-by": "publisher",
      "DOI": "10.1016/0921-4526(94)00655-F"
    },
    {
      "key": "S0883769400008721_ref013",
      "doi-asserted-by": "publisher",
      "DOI": "10.1103/PhysRevLett.86.5325"
    },
    {
      "key": "S0883769400008721_ref017",
      "doi-asserted-by": "publisher",
      "DOI": "10.1063/1.1841951"
    },
    {
      "key": "S0883769400008721_ref019",
      "doi-asserted-by": "publisher",
      "DOI": "10.1021/ja055754y"
    },
    {
      "key": "S0883769400008721_ref008",
      "doi-asserted-by": "publisher",
      "DOI": "10.1103/PhysRevLett.85.776"
    },
    {
      "key": "S0883769400008721_ref015",
      "doi-asserted-by": "publisher",
      "DOI": "10.1016/j.susc.2004.01.025"
    },
    {
      "key": "S0883769400008721_ref018",
      "doi-asserted-by": "publisher",
      "DOI": "10.1116/1.578531"
    },
    {
      "key": "S0883769400008721_ref005",
      "doi-asserted-by": "publisher",
      "DOI": "10.1103/PhysRevB.61.213"
    },
    {
      "key": "S0883769400008721_ref014",
      "doi-asserted-by": "publisher",
      "DOI": "10.1103/PhysRevLett.95.255505"
    },
    {
      "key": "S0883769400008721_ref028",
      "doi-asserted-by": "crossref",
      "first-page": "1",
      "DOI": "10.1080/01614949208021918",
      "volume": "34",
      "author": "Gai",
      "year": "1992",
      "journal-title": "Cat. Rev. Sci. Eng."
    },
    {
      "key": "S0883769400008721_ref029",
      "doi-asserted-by": "publisher",
      "DOI": "10.1016/j.ultramic.2006.01.006"
    },
    {
      "key": "S0883769400008721_ref010",
      "doi-asserted-by": "publisher",
      "DOI": "10.1016/j.surfrep.2005.03.002"
    },
    {
      "key": "S0883769400008721_ref031",
      "doi-asserted-by": "publisher",
      "DOI": "10.1126/science.1082146"
    },
    {
      "key": "S0883769400008721_ref009",
      "doi-asserted-by": "publisher",
      "DOI": "10.1016/S1381-1169(97)00270-7"
    },
    {
      "key": "S0883769400008721_ref012",
      "doi-asserted-by": "publisher",
      "DOI": "10.1016/j.susc.2006.05.030"
    },
    {
      "key": "S0883769400008721_ref022",
      "doi-asserted-by": "crossref",
      "first-page": "133",
      "DOI": "10.1016/S0360-0564(06)51004-1",
      "volume": "51",
      "author": "Rupprechter",
      "year": "2007",
      "journal-title": "Adv. Catal."
    },
    {
      "key": "S0883769400008721_ref023",
      "doi-asserted-by": "publisher",
      "DOI": "10.1039/b504027b"
    },
    {
      "key": "S0883769400008721_ref025",
      "doi-asserted-by": "publisher",
      "DOI": "10.1016/0920-5861(91)85023-2"
    }
  ],
  "container-title": "MRS Bulletin",
  "original-title": [],
  "language": "en",
  "link": [
    {
      "URL": "https://www.cambridge.org/core/services/aop-cambridge-core/content/view/S0883769400008721",
      "content-type": "unspecified",
      "content-version": "vor",
      "intended-application": "similarity-checking"
    }
  ],
  "deposited": {
    "date-parts": [
      [
        2024,
        4,
        3
      ]
    ],
    "date-time": "2024-04-03T19:21:17Z",
    "timestamp": 1712172077000
  },
  "score": 1,
  "resource": {
    "primary": {
      "URL": "http://link.springer.com/10.1557/mrs2007.208"
    }
  },
  "subtitle": [],
  "short-title": [],
  "issued": {
    "date-parts": [
      [
        2007,
        12
      ]
    ]
  },
  "references-count": 31,
  "journal-issue": {
    "issue": "12",
    "published-print": {
      "date-parts": [
        [
          2007,
          12
        ]
      ]
    }
  },
  "alternative-id": [
    "S0883769400008721"
  ],
  "URL": "http://dx.doi.org/10.1557/mrs2007.208",
  "relation": {},
  "ISSN": [
    "0883-7694",
    "1938-1425"
  ],
  "subject": [],
  "container-title-short": "MRS Bull.",
  "published": {
    "date-parts": [
      [
        2007,
        12
      ]
    ]
  }
}