DOI: 10.1126/science.260.5104.71. Evidence for Photochemical Formation of H 2 O 2 and Oxidation of SO 2 in Authentic Fog Water

Evidence for Photochemical Formation of H 2 O 2 and Oxidation of SO 2 in Authentic Fog Water

10.1126/science.260.5104.71

Crossref journal-article

American Association for the Advancement of Science (AAAS)

Science (221)

Abstract

When samples of rain and fog water were exposed to ultraviolet and visible light, reactive transients such as hydrogen peroxide were formed and dissolved organic matter and sulfur dioxide were depleted. These results, in conjunction with those from previous studies, imply that dissolved organic compounds and transition metals such as iron ions are involved in the photochemical formation of hydrogen peroxide and other photooxidants in atmospheric waters.

Bibliography

Zuo, Y., & HoignÃ©, J. (1993). Evidence for Photochemical Formation of H 2 O 2 and Oxidation of SO 2 in Authentic Fog Water. Science, 260(5104), 71â73.

Authors 2

Yuegang Zuo (first)
Jürg Hoigné (additional)

References 32 Referenced 147

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BALTENSPERGER, U, DETERMINATION OF MONO-VALENT AND DIVALENT-CATIONS AND ANIONS IN SMALL FOG SAMPLES BY ION CHROMATOGRAPHY, JOURNAL OF CHROMATOGRAPHY 439: 121 (1988). (10.1016/S0021-9673(01)81680-0) / JOURNAL OF CHROMATOGRAPHY (1988)
10.1038/344419a0
CALVERT, J.G., CHEMICAL MECHANISMS OF ACID GENERATION IN THE TROPOSPHERE, NATURE 317: 27 (1985). (10.1038/317027a0) / NATURE (1985)
CHAMEIDES, W.L., THE FREE-RADICAL CHEMISTRY OF CLOUD DROPLETS AND ITS IMPACT UPON THE COMPOSITION OF RAIN, JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS AND ATMOSPHERES 87: 4863 (1982). (10.1029/JC087iC07p04863) / JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS AND ATMOSPHERES (1982)
CHANDLER, A.S., MEASUREMENTS OF H2O2 AND SO2 IN CLOUDS AND ESTIMATES OF THEIR REACTION-RATE, NATURE 336: 562 (1988). (10.1038/336562a0) / NATURE (1988)
Cooper W. J. Aquatic Humic Substances: Influence on Fate and Treatment of Pollutants (1989).
COOPER, W.J., PHOTOCHEMICAL FORMATION OF HYDROGEN-PEROXIDE IN SURFACE AND GROUND WATERS EXPOSED TO SUNLIGHT, SCIENCE 220: 711 (1983). (10.1126/science.220.4598.711) / SCIENCE (1983)
FAUST, B. C., ATMOSPHERIC ENVIRONMENT PART A-GENERAL TOPICS 24: 79 (1990). (10.1016/0960-1686(90)90443-Q) / ATMOSPHERIC ENVIRONMENT PART A-GENERAL TOPICS (1990)
GERVAT, G.P., FIELD EVIDENCE FOR THE OXIDATION OF SO2 BY H2O2 IN CAP CLOUDS, NATURE 333: 241 (1988). (10.1038/333241a0) / NATURE (1988)
GRAEDEL, T. E., JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 91: 5205 (1986). (10.1029/JD091iD04p05205) / JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES (1986)
GRAEDEL, T.E., INFLUENCE OF TRANSITION-METAL COMPLEXES ON ATMOSPHERIC DROPLET ACIDITY, NATURE 317: 240 (1985). (10.1038/317240a0) / NATURE (1985)
HOFFMANN, M.R., KINETICS OF OXIDATION OF SULFITE BY HYDROGEN-PEROXIDE IN ACIDIC SOLUTION, JOURNAL OF PHYSICAL CHEMISTRY 79: 2096 (1975). (10.1021/j100587a005) / JOURNAL OF PHYSICAL CHEMISTRY (1975)
Hoigne, J., Aquatic and Surface Photochemistry: CH13 (1993). / Aquatic and Surface Photochemistry (1993)
JACOB, D.J., INSTRUMENT TO COLLECT FOGWATER FOR CHEMICAL-ANALYSIS, REVIEW OF SCIENTIFIC INSTRUMENTS 56: 1291 (1985). (10.1063/1.1137995) / REVIEW OF SCIENTIFIC INSTRUMENTS (1985)
JOHNSON, C.A., CASE-STUDIES ON THE CHEMICAL-COMPOSITION OF FOGWATER - THE INFLUENCE OF LOCAL GASEOUS EMISSIONS, ATMOSPHERIC ENVIRONMENT 21: 2365 (1987). (10.1016/0004-6981(87)90371-4) / ATMOSPHERIC ENVIRONMENT (1987)
KAWAMURA, K, INTERNATIONAL JOURNAL OF ENVIRONMENTAL ANALYTICAL CHEMISTRY 19: 175 (1985). (10.1080/03067318508077028) / INTERNATIONAL JOURNAL OF ENVIRONMENTAL ANALYTICAL CHEMISTRY (1985)
LELIEVELD, J, INFLUENCES OF CLOUD PHOTOCHEMICAL PROCESSES ON TROPOSPHERIC OZONE, NATURE 343: 227 (1990). (10.1038/343227a0) / NATURE (1990)
MCELROY, W.J., SOURCES OF HYDROGEN-PEROXIDE IN CLOUDWATER, ATMOSPHERIC ENVIRONMENT 20: 427 (1986). (10.1016/0004-6981(86)90082-X) / ATMOSPHERIC ENVIRONMENT (1986)
NORTON, R.B., TROPOSPHERIC OXALATE, GEOPHYSICAL RESEARCH LETTERS 10: 517 (1983). (10.1029/GL010i007p00517) / GEOPHYSICAL RESEARCH LETTERS (1983)
PEHKONEN, S, EOS 72: 108 (1991). / EOS (1991)
PENKETT, S.A., IMPORTANCE OF ATMOSPHERIC OZONE AND HYDROGEN-PEROXIDE IN OXIDIZING SULFUR-DIOXIDE IN CLOUD AND RAINWATER, ATMOSPHERIC ENVIRONMENT 13: 123 (1979). (10.1016/0004-6981(79)90251-8) / ATMOSPHERIC ENVIRONMENT (1979)
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STURZENEGGER V THESIS SWISS FEDERAL (1989).
WEINSTEINLLOYD, J, LOW-INTENSITY RADIOLYSIS STUDY OF FREE-RADICAL REACTIONS IN CLOUDWATER - H2O2 PRODUCTION AND DESTRUCTION, ENVIRONMENTAL SCIENCE & TECHNOLOGY 25: 791 (1991). (10.1021/es00016a027) / ENVIRONMENTAL SCIENCE & TECHNOLOGY (1991)
WESCHLER, C. J., JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 91: 5189 (1986). (10.1029/JD091iD04p05189) / JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES (1986)
ZEPP, R.G., HYDROXYL RADICAL FORMATION IN AQUEOUS REACTIONS (PH 3-8) OF IRON(II) WITH HYDROGEN-PEROXIDE - THE PHOTO-FENTON REACTION, ENVIRONMENTAL SCIENCE & TECHNOLOGY 26: 313 (1992). (10.1021/es00026a011) / ENVIRONMENTAL SCIENCE & TECHNOLOGY (1992)
ZUO, Y, EAWAG JAHRESBER 4: 31 (1990). / EAWAG JAHRESBER (1990)
ZUO, Y, FORMATION OF HYDROGEN-PEROXIDE AND DEPLETION OF OXALIC-ACID IN ATMOSPHERIC WATER BY PHOTOLYSIS OF IRON(III) OXALATO COMPLEXES, ENVIRONMENTAL SCIENCE & TECHNOLOGY 26: 1014 (1992). (10.1021/es00029a022) / ENVIRONMENTAL SCIENCE & TECHNOLOGY (1992)
ZUO Y THESIS SWISS FEDERAL (1992).

Dates

Type	When
Created	18 years, 10 months ago (Oct. 5, 2006, 7:05 p.m.)
Deposited	1 year, 7 months ago (Jan. 12, 2024, 5:59 p.m.)
Indexed	4 weeks, 1 day ago (July 28, 2025, 2:45 a.m.)
Issued	32 years, 4 months ago (April 2, 1993)
Published	32 years, 4 months ago (April 2, 1993)
Published Print	32 years, 4 months ago (April 2, 1993)

Funders 0

None

BibTeX

@article{Zuo_1993, title={Evidence for Photochemical Formation of H 2 O 2 and Oxidation of SO 2 in Authentic Fog Water}, volume={260}, ISSN={1095-9203}, url={http://dx.doi.org/10.1126/science.260.5104.71}, DOI={10.1126/science.260.5104.71}, number={5104}, journal={Science}, publisher={American Association for the Advancement of Science (AAAS)}, author={Zuo, Yuegang and Hoigné, Jürg}, year={1993}, month=apr, pages={71–73} }

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