Crossref journal-article
American Association for the Advancement of Science (AAAS)
Science (221)
Abstract

The average worldwide tropospheric mixing ratio of methane has increased by 11% from 1.52 parts per million by volume (ppmv) in January 1978 to 1.684 ppmv in September 1987, for an increment of 0.016 ± 0.001 ppmv per year. Within the limits of our measurements, the global tropospheric mixing ratio for methane over the past decade is consistent either with a linear growth rate of 0.016 ± 0.001 ppmv per year or with a slight lessening of the rate of growth over the past 5 years. No indications were found of an effect of the El Niño-Southern Oscillation-El Chichon events of 1982-83 on total global methane, although severe reductions were reported in the Pacific Northwest during that time period. The growth in tropospheric methane may have increased the water concentration in the stratosphere by as much as 28% since the 1940s and 45% over the past two centuries and thus could have increased the mass of precipitable water available for formation of polar stratospheric clouds.

Bibliography

Blake, D. R., & Rowland, F. S. (1988). Continuing Worldwide Increase in Tropospheric Methane, 1978 to 1987. Science, 239(4844), 1129–1131.

Authors 2
  1. Donald R. Blake (first)
  2. F. Sherwood Rowland (additional)
References 42 Referenced 390
  1. WMO16 WORLD MET ORG (1986).
  2. BLAKE, D.R., GLOBAL INCREASE IN ATMOSPHERIC METHANE CONCENTRATIONS BETWEEN 1978 AND 1980, GEOPHYSICAL RESEARCH LETTERS 9: 477 (1982). (10.1029/GL009i004p00477) / GEOPHYSICAL RESEARCH LETTERS (1982)
  3. BLAKE, D.R., METHANE CONCENTRATIONS AND SOURCE STRENGTHS IN URBAN LOCATIONS, GEOPHYSICAL RESEARCH LETTERS 11: 1211 (1984). (10.1029/GL011i012p01211) / GEOPHYSICAL RESEARCH LETTERS (1984)
  4. BLAKE, D.R., WORLDWIDE INCREASE IN TROPOSPHERIC METHANE, 1978-1983, JOURNAL OF ATMOSPHERIC CHEMISTRY 4: 43 (1986). (10.1007/BF00053772) / JOURNAL OF ATMOSPHERIC CHEMISTRY (1986)
  5. BLAKE, D.R., GLOBAL ATMOSPHERIC CONCENTRATIONS AND SOURCE STRENGTH OF ETHANE, NATURE 321: 231 (1986). (10.1038/321231a0) / NATURE (1986)
  6. CRAIG, H, METHANE - THE RECORD IN POLAR ICE CORES, GEOPHYSICAL RESEARCH LETTERS 9: 1221 (1982). (10.1029/GL009i011p01221) / GEOPHYSICAL RESEARCH LETTERS (1982)
  7. 10.1038/319109a0
  8. EHHALT, D.H., ON THE TEMPORAL INCREASE OF TROPOSPHERIC CH4, JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS AND ATMOSPHERES 88: 8442 (1983). (10.1029/JC088iC13p08442) / JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS AND ATMOSPHERES (1983)
  9. EHHALT, D.H., SOURCES AND SINKS OF ATMOSPHERIC METHANE, PURE AND APPLIED GEOPHYSICS 116: 452 (1978). (10.1007/BF01636899) / PURE AND APPLIED GEOPHYSICS (1978)
  10. FARMAN, J.C., LARGE LOSSES OF TOTAL OZONE IN ANTARCTICA REVEAL SEASONAL CLOX/NOX INTERACTION, NATURE 315: 207 (1985). (10.1038/315207a0) / NATURE (1985)
  11. FRASER, P.J., TRENDS OF ATMOSPHERIC METHANE IN THE SOUTHERN-HEMISPHERE, GEOPHYSICAL RESEARCH LETTERS 8: 1063 (1981). (10.1029/GL008i010p01063) / GEOPHYSICAL RESEARCH LETTERS (1981)
  12. FRASER, P.J., TROPOSPHERIC METHANE IN THE MID-LATITUDES OF THE SOUTHERN-HEMISPHERE, JOURNAL OF ATMOSPHERIC CHEMISTRY 1: 125 (1984). (10.1007/BF00053835) / JOURNAL OF ATMOSPHERIC CHEMISTRY (1984)
  13. FRASER, P.J., METHANE, CARBON-MONOXIDE AND METHYLCHLOROFORM IN THE SOUTHERN-HEMISPHERE, JOURNAL OF ATMOSPHERIC CHEMISTRY 4: 3 (1986). (10.1007/BF00053771) / JOURNAL OF ATMOSPHERIC CHEMISTRY (1986)
  14. HOFMANN, D.J., BALLOON-BORNE OBSERVATIONS OF THE DEVELOPMENT AND VERTICAL STRUCTURE OF THE ANTARCTIC OZONE HOLE IN 1986, NATURE 326: 59 (1987). (10.1038/326059a0) / NATURE (1987)
  15. JONES, R.L., THE WATER-VAPOR BUDGET OF THE STRATOSPHERE STUDIED USING LIMS AND SAMS SATELLITE DATA, QUARTERLY JOURNAL OF THE ROYAL METEOROLOGICAL SOCIETY 112: 1127 (1986). (10.1002/qj.49711247412) / QUARTERLY JOURNAL OF THE ROYAL METEOROLOGICAL SOCIETY (1986)
  16. KHALIL, MAK, ANTARCTIC JOURNAL OF THE UNITED STATES 19: 204 (1984). / ANTARCTIC JOURNAL OF THE UNITED STATES (1984)
  17. KHALIL, MAK, SOURCES, SINKS, AND SEASONAL CYCLES OF ATMOSPHERIC METHANE, JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS AND ATMOSPHERES 88: 5131 (1983). (10.1029/JC088iC09p05131) / JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS AND ATMOSPHERES (1983)
  18. 10.1126/science.232.4746.56
  19. LEVINE, J.S., THE PHOTOCHEMISTRY OF METHANE AND CARBON-MONOXIDE IN THE TROPOSPHERE IN 1950 AND 1985, NATURE 318: 254 (1985). (10.1038/318254a0) / NATURE (1985)
  20. MAKIDE, Y, TROPOSPHERIC CONCENTRATIONS OF METHYLCHLOROFORM, CH3CCL3, IN JANUARY 1978 AND ESTIMATES OF THE ATMOSPHERIC RESIDENCE TIMES FOR HYDROHALOCARBONS, PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA-PHYSICAL SCIENCES 78: 5933 (1981). / PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA-PHYSICAL SCIENCES (1981)
  21. MATTHEWS, E, GLOBAL BIOGEOCHEMICA 1: 61 (1987). (10.1029/GB001i001p00061) / GLOBAL BIOGEOCHEMICA (1987)
  22. MAYER, E.W., METHANE - INTER-HEMISPHERIC CONCENTRATION GRADIENT AND ATMOSPHERIC RESIDENCE TIME, PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA-PHYSICAL SCIENCES 79: 1366 (1982). / PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA-PHYSICAL SCIENCES (1982)
  23. MCELROY, M.B., REDUCTIONS OF ANTARCTIC OZONE DUE TO SYNERGISTIC INTERACTIONS OF CHLORINE AND BROMINE, NATURE 321: 759 (1986). (10.1038/321759a0) / NATURE (1986)
  24. MOLINA, L.T., PRODUCTION OF CL2O2 FROM THE SELF-REACTION OF THE CIO RADICAL, JOURNAL OF PHYSICAL CHEMISTRY 91: 433 (1987). (10.1021/j100286a035) / JOURNAL OF PHYSICAL CHEMISTRY (1987)
  25. PEARMAN, G.I., EVIDENCE OF CHANGING CONCENTRATIONS OF ATMOSPHERIC CO2, N2O AND CH4 FROM AIR BUBBLES IN ANTARCTIC ICE, NATURE 320: 248 (1986). (10.1038/320248a0) / NATURE (1986)
  26. RAMANATHAN, V, TRACE GAS TRENDS AND THEIR POTENTIAL ROLE IN CLIMATE CHANGE, JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 90: 5547 (1985). (10.1029/JD090iD03p05547) / JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES (1985)
  27. RASMUSSEN, R.A., ATMOSPHERIC METHANE (CH4) - TRENDS AND SEASONAL CYCLES, JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS AND ATMOSPHERES 86: 9826 (1981). (10.1029/JC086iC10p09826) / JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS AND ATMOSPHERES (1981)
  28. RASMUSSEN, R.A., ATMOSPHERIC METHANE IN THE RECENT AND ANCIENT ATMOSPHERES - CONCENTRATIONS, TRENDS, AND INTERHEMISPHERIC GRADIENT, JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 89: 11599 (1984). (10.1029/JD089iD07p11599) / JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES (1984)
  29. RINSLAND, C.P., CONCENTRATION OF METHANE IN THE TROPOSPHERE DEDUCED FROM 1951 INFRARED SOLAR SPECTRA, NATURE 318: 245 (1985). (10.1038/318245a0) / NATURE (1985)
  30. RINSLAND, C.P., FREE TROPOSPHERIC CARBON-MONOXIDE CONCENTRATIONS IN 1950 AND 1951 DEDUCED FROM INFRARED TOTAL COLUMN AMOUNT MEASUREMENTS, NATURE 318: 250 (1985). (10.1038/318250a0) / NATURE (1985)
  31. ROBBINS, R.C., ANALYSIS OF ANCIENT ATMOSPHERES, JOURNAL OF GEOPHYSICAL RESEARCH 78: 5341 (1973). (10.1029/JC078i024p05341) / JOURNAL OF GEOPHYSICAL RESEARCH (1973)
  32. ROBINSON, E, ATMOSPHERIC TRACE GAS MEASUREMENTS AT PALMER STATION, ANTARCTICA - 1982-83, JOURNAL OF ATMOSPHERIC CHEMISTRY 2: 65 (1984). (10.1007/BF00127263) / JOURNAL OF ATMOSPHERIC CHEMISTRY (1984)
  33. ROWLAND, F.S., THE HYDROLYSIS OF CHLORINE NITRATE AND ITS POSSIBLE ATMOSPHERIC SIGNIFICANCE, JOURNAL OF PHYSICAL CHEMISTRY 90: 1985 (1986). (10.1021/j100401a001) / JOURNAL OF PHYSICAL CHEMISTRY (1986)
  34. ROWLAND, F.S., METHANE AND CHLOROCARBONS IN THE EARTHS ATMOSPHERE, ORIGINS OF LIFE AND EVOLUTION OF THE BIOSPHERE 15: 279 (1985). (10.1007/BF01808174) / ORIGINS OF LIFE AND EVOLUTION OF THE BIOSPHERE (1985)
  35. ROWLAND, F.S., WMO16 WORLD MET ORG: 13 (1985). / WMO16 WORLD MET ORG (1985)
  36. ROWLAND, F.S., WMO16 WORLD MET ORG: 33 (1985). / WMO16 WORLD MET ORG (1985)
  37. SOLOMON, S, ON THE DEPLETION OF ANTARCTIC OZONE, NATURE 321: 755 (1986). (10.1038/321755a0) / NATURE (1986)
  38. 10.1126/science.229.4720.1386
  39. 10.1007/BF00048857
  40. STEPHENS, E.R., TROPOSHERIC METHANE - CONCENTRATIONS BETWEEN 1963 AND 1970, JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 90: 3076 (1985). / JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES (1985)
  41. STOLARSKI, R.S., NIMBUS-7 SATELLITE MEASUREMENTS OF THE SPRINGTIME ANTARCTIC OZONE DECREASE, NATURE 322: 808 (1986). (10.1038/322808a0) / NATURE (1986)
  42. THOMPSON, A.M., POSSIBLE PERTURBATIONS TO ATMOSPHERIC CO, CH4, AND OH, JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 91: 10853 (1986). (10.1029/JD091iD10p10853) / JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES (1986)
Dates
Type When
Created 18 years, 10 months ago (Oct. 5, 2006, 5:21 p.m.)
Deposited 1 year, 7 months ago (Jan. 12, 2024, 11:51 a.m.)
Indexed 2 weeks ago (Aug. 12, 2025, 5:31 p.m.)
Issued 37 years, 5 months ago (March 4, 1988)
Published 37 years, 5 months ago (March 4, 1988)
Published Print 37 years, 5 months ago (March 4, 1988)
Funders 0

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@article{Blake_1988, title={Continuing Worldwide Increase in Tropospheric Methane, 1978 to 1987}, volume={239}, ISSN={1095-9203}, url={http://dx.doi.org/10.1126/science.239.4844.1129}, DOI={10.1126/science.239.4844.1129}, number={4844}, journal={Science}, publisher={American Association for the Advancement of Science (AAAS)}, author={Blake, Donald R. and Rowland, F. Sherwood}, year={1988}, month=mar, pages={1129–1131} }