DOI: 10.1073/pnas.1501911112. Assessing the role of static length scales behind glassy dynamics in polydisperse hard disks

Assessing the role of static length scales behind glassy dynamics in polydisperse hard disks

10.1073/pnas.1501911112

Crossref journal-article

Proceedings of the National Academy of Sciences

Proceedings of the National Academy of Sciences (341)

Abstract

Significance The origin of dynamical slowing down toward glass transition is a fundamental unsolved problem in condensed matter physics. A crucial question is whether this slowing down has a structural origin. Recently, a method to detect hidden order within the fluid was proposed, based on the idea that freezing a fraction of the particles in a system causes a transition akin to glass transition. Here, we show that a glass former, polydisperse hard disks, has a strong increase of structural order, well correlated with slow dynamics, which goes undetected by the pinning method. This casts doubt on the order-agnostic qualities of the pinning length scale and keeps static length scales in the race for plausible explanations of the glass transition problem.

Bibliography

Russo, J., & Tanaka, H. (2015). Assessing the role of static length scales behind glassy dynamics in polydisperse hard disks. Proceedings of the National Academy of Sciences, 112(22), 6920â6924.

Authors 2

John Russo (first)
Hajime Tanaka (additional)

References 38 Referenced 52

Dates

Type	When
Created	10 years, 3 months ago (May 18, 2015, 10:50 p.m.)
Deposited	3 years, 4 months ago (April 13, 2022, 12:30 a.m.)
Indexed	6 months, 1 week ago (Feb. 21, 2025, 3:50 a.m.)
Issued	10 years, 3 months ago (May 18, 2015)
Published	10 years, 3 months ago (May 18, 2015)
Published Online	10 years, 3 months ago (May 18, 2015)
Published Print	10 years, 2 months ago (June 2, 2015)

Funders 2

Japan Society for the Promotion of Science 10.13039/501100001691
Region: Asia
gov (National government)
Labels6
1. KAKENHI
2. 日本学術振興会
3. Gakushin
4. JSPS KAKEN
5. JSPS Grants-in-Aid for Scientific Research
6. JSPS
Awards1
1. 25000002
Japan Society for the Promotion of Science 10.13039/501100001691
Region: Asia
gov (National government)
Labels6
1. KAKENHI
2. 日本学術振興会
3. Gakushin
4. JSPS KAKEN
5. JSPS Grants-in-Aid for Scientific Research
6. JSPS
Awards1
1. 21224011

BibTeX

@article{Russo_2015, title={Assessing the role of static length scales behind glassy dynamics in polydisperse hard disks}, volume={112}, ISSN={1091-6490}, url={http://dx.doi.org/10.1073/pnas.1501911112}, DOI={10.1073/pnas.1501911112}, number={22}, journal={Proceedings of the National Academy of Sciences}, publisher={Proceedings of the National Academy of Sciences}, author={Russo, John and Tanaka, Hajime}, year={2015}, month=may, pages={6920–6924} }

JSON

{
  "indexed": {
    "date-parts": [
      [
        2025,
        2,
        21
      ]
    ],
    "date-time": "2025-02-21T08:50:09Z",
    "timestamp": 1740127809726,
    "version": "3.37.3"
  },
  "reference-count": 38,
  "publisher": "Proceedings of the National Academy of Sciences",
  "issue": "22",
  "license": [
    {
      "start": {
        "date-parts": [
          [
            2015,
            11,
            18
          ]
        ],
        "date-time": "2015-11-18T00:00:00Z",
        "timestamp": 1447804800000
      },
      "content-version": "vor",
      "delay-in-days": 184,
      "URL": "http://www.pnas.org/site/misc/userlicense.xhtml"
    }
  ],
  "funder": [
    {
      "DOI": "10.13039/501100001691",
      "name": "Japan Society for the Promotion of Science",
      "doi-asserted-by": "publisher",
      "award": [
        "25000002"
      ],
      "id": [
        {
          "id": "10.13039/501100001691",
          "id-type": "DOI",
          "asserted-by": "publisher"
        }
      ]
    },
    {
      "DOI": "10.13039/501100001691",
      "name": "Japan Society for the Promotion of Science",
      "doi-asserted-by": "publisher",
      "award": [
        "21224011"
      ],
      "id": [
        {
          "id": "10.13039/501100001691",
          "id-type": "DOI",
          "asserted-by": "publisher"
        }
      ]
    }
  ],
  "content-domain": {
    "domain": [
      "www.pnas.org"
    ],
    "crossmark-restriction": true
  },
  "published-print": {
    "date-parts": [
      [
        2015,
        6,
        2
      ]
    ]
  },
  "abstract": "<jats:title>Significance</jats:title>\n          <jats:p>The origin of dynamical slowing down toward glass transition is a fundamental unsolved problem in condensed matter physics. A crucial question is whether this slowing down has a structural origin. Recently, a method to detect hidden order within the fluid was proposed, based on the idea that freezing a fraction of the particles in a system causes a transition akin to glass transition. Here, we show that a glass former, polydisperse hard disks, has a strong increase of structural order, well correlated with slow dynamics, which goes undetected by the pinning method. This casts doubt on the order-agnostic qualities of the pinning length scale and keeps static length scales in the race for plausible explanations of the glass transition problem.</jats:p>",
  "DOI": "10.1073/pnas.1501911112",
  "type": "journal-article",
  "created": {
    "date-parts": [
      [
        2015,
        5,
        19
      ]
    ],
    "date-time": "2015-05-19T02:50:56Z",
    "timestamp": 1432003856000
  },
  "page": "6920-6924",
  "update-policy": "https://doi.org/10.1073/pnas.cm10313",
  "source": "Crossref",
  "is-referenced-by-count": 52,
  "title": "Assessing the role of static length scales behind glassy dynamics in polydisperse hard disks",
  "prefix": "10.1073",
  "volume": "112",
  "author": [
    {
      "given": "John",
      "family": "Russo",
      "sequence": "first",
      "affiliation": [
        {
          "name": "Department of Fundamental Engineering, Institute of Industrial Science, University of Tokyo, Tokyo 153-8505, Japan"
        }
      ]
    },
    {
      "given": "Hajime",
      "family": "Tanaka",
      "sequence": "additional",
      "affiliation": [
        {
          "name": "Department of Fundamental Engineering, Institute of Industrial Science, University of Tokyo, Tokyo 153-8505, Japan"
        }
      ]
    }
  ],
  "member": "341",
  "published-online": {
    "date-parts": [
      [
        2015,
        5,
        18
      ]
    ]
  },
  "reference": [
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_1_2",
      "DOI": "10.1103/PhysRevLett.79.2827"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_2_2",
      "DOI": "10.1103/PhysRevE.58.3515"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_3_2",
      "DOI": "10.1103/RevModPhys.83.587"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_4_2",
      "DOI": "10.1126/science.1166665"
    },
    {
      "doi-asserted-by": "crossref",
      "unstructured": "CP Royall SR Williams The role of local structure in dynamical arrest. arXiv:1405.5691. (2014).",
      "key": "e_1_3_3_5_2",
      "DOI": "10.1016/j.physrep.2014.11.004"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_6_2",
      "DOI": "10.1063/1.4790138"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_7_2",
      "DOI": "10.1103/PhysRevA.40.1045"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_8_2",
      "DOI": "10.1146/annurev.physchem.58.032806.104653"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_9_2",
      "DOI": "10.1103/RevModPhys.82.789"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_10_2",
      "DOI": "10.1140/epje/i2012-12113-y"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_11_2",
      "DOI": "10.1038/nmat2634"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_12_2",
      "DOI": "10.1103/PhysRevLett.99.215701"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_13_2",
      "DOI": "10.1088/0953-8984/23/19/194121"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_14_2",
      "DOI": "10.1103/PhysRevLett.108.035701"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_15_2",
      "DOI": "10.1016/j.physrep.2009.03.003"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_16_2",
      "DOI": "10.1063/1.4720477"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_17_2",
      "DOI": "10.1073/pnas.1111582109"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_18_2",
      "DOI": "10.1063/1.4790400"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_19_2",
      "DOI": "10.1103/PhysRevLett.110.245702"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_20_2",
      "DOI": "10.1073/pnas.1222848110"
    },
    {
      "doi-asserted-by": "crossref",
      "unstructured": "S Chakrabarty S Karmakar C Dasgupta Phase diagram of glass forming liquids with randomly pinned particles. arXiv:1404.2701. (2014).",
      "key": "e_1_3_3_21_2",
      "DOI": "10.1038/srep12577"
    },
    {
      "doi-asserted-by": "crossref",
      "unstructured": "M Ozawa W Kob A Ikeda K Miyazaki Equilibrium phase diagram of a randomly pinned glass-former. arXiv:1412.4911. (2014).",
      "key": "e_1_3_3_22_2",
      "DOI": "10.1073/pnas.1500730112"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_23_2",
      "DOI": "10.1103/PhysRevE.87.042305"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_24_2",
      "DOI": "10.1103/PhysRevLett.113.157801"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_25_2",
      "DOI": "10.1007/s10955-006-9175-y"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_26_2",
      "DOI": "10.1103/PhysRevE.88.012122"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_27_2",
      "DOI": "10.1103/PhysRevLett.108.225506"
    },
    {
      "doi-asserted-by": "crossref",
      "unstructured": "E Flenner H Staley G Szamel Universal features of dynamic heterogeneity in supercooled liquids. arXiv:1310.1029. (2013).",
      "key": "e_1_3_3_28_2",
      "DOI": "10.1103/PhysRevLett.112.097801"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_29_2",
      "DOI": "10.1103/PhysRevLett.111.165701"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_30_2",
      "DOI": "10.1103/PhysRevE.85.011102"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_31_2",
      "DOI": "10.1038/nphys1050"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_32_2",
      "DOI": "10.1063/1.4769981"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_33_2",
      "DOI": "10.1103/PhysRevE.88.042304"
    },
    {
      "doi-asserted-by": "crossref",
      "unstructured": "W Kob D Coslovich Non-linear dynamic response of glass-forming liquids to random pinning. arXiv:1403.3519. (2014).",
      "key": "e_1_3_3_34_2",
      "DOI": "10.1103/PhysRevE.90.052305"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_35_2",
      "DOI": "10.1103/PhysRevE.80.056704"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_36_2",
      "DOI": "10.1103/PhysRevLett.107.155704"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_37_2",
      "DOI": "10.1002/jcc.21915"
    },
    {
      "doi-asserted-by": "publisher",
      "key": "e_1_3_3_38_2",
      "DOI": "10.1103/PhysRevLett.93.135701"
    }
  ],
  "container-title": "Proceedings of the National Academy of Sciences",
  "original-title": [],
  "language": "en",
  "link": [
    {
      "URL": "http://www.pnas.org/syndication/doi/10.1073/pnas.1501911112",
      "content-type": "unspecified",
      "content-version": "vor",
      "intended-application": "syndication"
    },
    {
      "URL": "https://pnas.org/doi/pdf/10.1073/pnas.1501911112",
      "content-type": "unspecified",
      "content-version": "vor",
      "intended-application": "similarity-checking"
    }
  ],
  "deposited": {
    "date-parts": [
      [
        2022,
        4,
        13
      ]
    ],
    "date-time": "2022-04-13T04:30:19Z",
    "timestamp": 1649824219000
  },
  "score": 1,
  "resource": {
    "primary": {
      "URL": "https://pnas.org/doi/full/10.1073/pnas.1501911112"
    }
  },
  "subtitle": [],
  "short-title": [],
  "issued": {
    "date-parts": [
      [
        2015,
        5,
        18
      ]
    ]
  },
  "references-count": 38,
  "journal-issue": {
    "issue": "22",
    "published-print": {
      "date-parts": [
        [
          2015,
          6,
          2
        ]
      ]
    }
  },
  "alternative-id": [
    "10.1073/pnas.1501911112"
  ],
  "URL": "http://dx.doi.org/10.1073/pnas.1501911112",
  "relation": {},
  "ISSN": [
    "0027-8424",
    "1091-6490"
  ],
  "subject": [],
  "container-title-short": "Proc. Natl. Acad. Sci. U.S.A.",
  "published": {
    "date-parts": [
      [
        2015,
        5,
        18
      ]
    ]
  },
  "assertion": [
    {
      "value": "2015-05-18",
      "order": 2,
      "name": "published",
      "label": "Published",
      "group": {
        "name": "publication_history",
        "label": "Publication History"
      }
    }
  ]
}