Crossref journal-article
AIP Publishing
Applied Physics Letters (317)
Abstract

We investigate valley exciton dynamics in MoSe2 monolayers in polarization- and time-resolved photoluminescence (PL) spectroscopy at 4 K. Following circularly polarized laser excitation, we record a low circular polarization degree of the PL of typically ≤5%. This is about 10 times lower than the polarization induced under comparable conditions in MoS2 and WSe2 monolayers. The evolution of the exciton polarization as a function of excitation laser energy and power is monitored in PL excitation experiments. Fast PL emission times are recorded for both the neutral exciton of ≤3 ps and for the charged exciton (trion) of 12 ps.

Bibliography

Wang, G., Palleau, E., Amand, T., Tongay, S., Marie, X., & Urbaszek, B. (2015). Polarization and time-resolved photoluminescence spectroscopy of excitons in MoSe2 monolayers. Applied Physics Letters, 106(11).

Authors 6
  1. G. Wang (first)
  2. E. Palleau (additional)
  3. T. Amand (additional)
  4. S. Tongay (additional)
  5. X. Marie (additional)
  6. B. Urbaszek (additional)
References 39 Referenced 142
  1. 10.1103/PhysRevLett.105.136805 / Phys. Rev. Lett. (2010)
  2. 10.1021/nl903868w / Nano Lett. (2010)
  3. 10.1038/nnano.2013.277 / Nat. Nanotechnol. (2014)
  4. 10.1103/PhysRevB.85.205302 / Phys. Rev. B (2012)
  5. 10.1103/PhysRevB.86.241201 / Phys. Rev. B (2012)
  6. 10.1103/PhysRevLett.113.026803 / Phys. Rev. Lett. (2014)
  7. 10.1038/nmat4061 / Nat. Mater. (2014)
  8. 10.1103/PhysRevLett.113.076802 / Phys. Rev. Lett. (2014)
  9. 10.1038/nature13734 / Nature (2014)
  10. 10.1038/ncomms2498 / Nat. Commun. (2013)
  11. 10.1038/srep06608 / Sci. Rep. (2014)
  12. 10.1103/PhysRevLett.114.097403 / Phys. Rev. Lett. (2015)
  13. 10.1038/nature12385 / Nature (2013)
  14. 10.1038/nphys2942 / Nat. Phys. (2014)
  15. 10.1103/PhysRevLett.108.196802 / Phys. Rev. Lett. (2012)
  16. 10.1038/ncomms1882 / Nat. Commun. (2012)
  17. 10.1038/nnano.2012.96 / Nat. Nanotechnol. (2012)
  18. 10.1103/PhysRevB.86.081301 / Phys. Rev. B (2012)
  19. 10.1063/1.4768299 / Appl. Phys. Lett. (2012)
  20. 10.1038/nnano.2013.151 / Nat. Nanotechnol. (2013)
  21. 10.1126/science.1250140 / Science (2014)
  22. 10.1038/nnano.2012.95 / Nat. Nanotechnol. (2012)
  23. 10.1073/pnas.1406960111 / Proc. Natl. Acad. Sci. U. S. A. (2014)
  24. 10.1103/PhysRevLett.112.216804 / Phys. Rev. Lett. (2014)
  25. 10.1039/C4NR03607G / Nanoscale (2014)
  26. 10.1103/PhysRevLett.112.047401 / Phys. Rev. Lett. (2014)
  27. 10.1103/PhysRevB.90.075413 / Phys. Rev. B (2014)
  28. 10.1088/2053-1583/1/1/011002 / 2D Mater. (2014)
  29. 10.1103/PhysRevLett.113.266804 / Phys. Rev. Lett. (2014)
  30. 10.1103/PhysRevLett.114.037401 / Phys. Rev. Lett. (2015)
  31. 10.1103/PhysRevB.89.201302 / Phys. Rev. B (2014)
  32. 10.1103/PhysRevB.89.205303 / Phys. Rev. B (2014)
  33. {'volume-title': 'Springer Series in Solid-State Science', 'year': '2008', 'key': '2023061800083029500_c33'} / Springer Series in Solid-State Science (2008)
  34. 10.1103/PhysRevB.90.161302 / Phys. Rev. B (2014)
  35. 10.1103/PhysRevB.47.15776 / Phys. Rev. B (1993)
  36. 10.1103/PhysRevB.88.085433 / Phys. Rev. B (2013)
  37. 10.1103/PhysRevB.88.245436 / Phys. Rev. B (2013)
  38. A. Kormanyos, G. Burkard, M. Gmitra, J. Fabian, V. Zolyomi, N. D. Drummond, and V. Fal'ko, e-print arXiv:1410.6666 (2014).
  39. G. Wang, L. Bouet, M. M. Glazov, T. Amand, E. L. Ivchenko, E. Palleau, X. Marie, and B. Urbaszek, e-print arXiv:1503.04105 (2015).
Dates
Type When
Created 10 years, 5 months ago (March 18, 2015, 2:11 p.m.)
Deposited 2 years, 2 months ago (June 17, 2023, 8:08 p.m.)
Indexed 5 days, 19 hours ago (Aug. 23, 2025, 9:51 p.m.)
Issued 10 years, 5 months ago (March 16, 2015)
Published 10 years, 5 months ago (March 16, 2015)
Published Online 10 years, 5 months ago (March 18, 2015)
Published Print 10 years, 5 months ago (March 16, 2015)
Funders 2
  1. European Research Council 10.13039/501100000781

    Region: Europe

    gov (National government)

    Labels1
    1. ERC
    Awards1
    1. 306719
  2. Agence Nationale de la Recherche 10.13039/501100001665

    Region: Europe

    gov (National government)

    Labels3
    1. French National Research Agency
    2. French National Agency for Research
    3. ANR

@article{Wang_2015, title={Polarization and time-resolved photoluminescence spectroscopy of excitons in MoSe2 monolayers}, volume={106}, ISSN={1077-3118}, url={http://dx.doi.org/10.1063/1.4916089}, DOI={10.1063/1.4916089}, number={11}, journal={Applied Physics Letters}, publisher={AIP Publishing}, author={Wang, G. and Palleau, E. and Amand, T. and Tongay, S. and Marie, X. and Urbaszek, B.}, year={2015}, month=mar }