Abstract
We investigate exciton dynamics in WSe2 bilayers in time-resolved photoluminescence (PL) spectroscopy. Fast PL emission times are recorded for both the direct exciton with τD ≲ 3 ps and the indirect optical transition with τI ≈ 25 ps. For temperatures between 4 to 150 K τI remains constant. Following polarized laser excitation, we observe for the direct exciton transition at the K point of the Brillouin zone efficient optical orientation and alignment during the short emission time τD. The evolution of the direct exciton polarization and intensity as a function of excitation laser energy is monitored in PL excitation experiments.
References
44
Referenced
50
10.1038/nature12385
/ Nature (2013)10.1038/nphys2942
/ Nat. Phys. (2014)10.1103/PhysRevLett.105.136805
/ Phys. Rev. Lett. (2010)10.1021/nl903868w
/ Nano Lett. (2010)10.1103/PhysRevLett.108.196802
/ Phys. Rev. Lett. (2012)10.1038/ncomms1882
/ Nat. Commun. (2012)10.1038/nnano.2012.96
/ Nat. Nanotechnol. (2012)10.1103/PhysRevB.86.081301
/ Phys. Rev. B (2012)10.1063/1.4768299
/ Appl. Phys. Lett. (2012)10.1038/nnano.2013.151
/ Nat. Nanotechnol. (2013)10.1126/science.1250140
/ Science (2014)10.1103/PhysRevB.85.205302
/ Phys. Rev. B (2012)10.1103/PhysRevB.86.241201
/ Phys. Rev. B (2012)10.1103/PhysRevLett.113.026803
/ Phys. Rev. Lett. (2014)10.1038/nmat4061
/ Nat. Mater. / Giant bandgap renormalization and excitonic effects in a monolayer transition metal dichalcogenide semiconductor10.1103/PhysRevLett.113.076802
/ Phys. Rev. Lett. (2014)10.1038/nature13734
/ Nature (2014)- G. Wang, X. Marie, I. Gerber, T. Amand, D. Lagarde, L. Bouet, M. Vidal, A. Balocchi, and B. Urbaszek, e-print arXiv:1404.0056 (2014).
10.1103/PhysRevLett.111.106801
/ Phys. Rev. Lett. (2013)10.1038/nnano.2013.277
/ Nat. Nanotechnol. (2014)10.1038/nphys2848
/ Nat. Phys. (2014)10.1073/pnas.1406960111
/ Proc. Natl. Acad. Sci. (2014)- Q. Liu, X. Zhang, and A. Zunger, e-print arXiv:1408.6001 (2014).
10.1103/PhysRevB.90.035437
/ Phys. Rev. B (2014)10.1063/1.3636402
/ Appl. Phys. Lett. (2011)10.1103/PhysRevLett.112.047401
/ Phys. Rev. Lett. (2014)10.1021/nn303973r
/ ACS Nano (2013)10.1021/nn405419h
/ ACS Nano (2013)10.1021/nl403742j
/ Nano Lett. (2014)10.1103/PhysRevB.90.075413
/ Phys. Rev. B (2014)- P. Rivera, J. R. Schaibley, A. M. Jones, J. S. Ross, S. Wu, G. Aivazian, P. Klement, N. J. Ghimire, J. Yan, D. G. Mandrus et al., e-print arXiv:1403.4985 (2014).
- Y. Yu, S. Hu, L. Su, L. Huang, Y. Liu, Z. Jin, A. A. Purezky, D. B. Geohegan, K. W. Kim, Y. Zhang et al., e-print arXiv:1403.6181 (2014).
10.1103/RevModPhys.85.79
/ Rev. Mod. Phys. (2013)10.1103/PhysRevB.87.165409
/ Phys. Rev. B (2013)10.1021/nn305275h
/ ACS Nano (2013)10.1021/nl403270k
/ Nano Lett. (2013)10.1103/PhysRevB.89.205311
/ Phys. Rev. B (2014){'first-page': '6', 'volume-title': 'Proceedings of the Sixth International Conference on Indium Phosphide and Related Materials, 1994', 'year': '1994', 'key': '2023062415552269200_c39'}
/ Proceedings of the Sixth International Conference on Indium Phosphide and Related Materials, 1994 (1994)10.1038/nphys2933
/ Nat. Phys. (2014)10.1038/nphys3105
/ Nat. Phys. / Direct observation of spin-polarized bulk bands in an inversion-symmetric semiconductor10.1103/PhysRevB.89.201302
/ Phys. Rev. B (2014)10.1103/PhysRevB.89.205303
/ Phys. Rev. B (2014)10.1103/PhysRevB.90.161302
/ Phys. Rev. B (2014)10.1038/ncomms5555
/ Nat. Commun. (2014)
Dates
Type | When |
---|---|
Created | 10 years, 10 months ago (Nov. 4, 2014, 8:31 p.m.) |
Deposited | 2 years, 2 months ago (June 24, 2023, 10:28 p.m.) |
Indexed | 4 weeks, 1 day ago (Aug. 6, 2025, 9:29 a.m.) |
Issued | 10 years, 10 months ago (Nov. 3, 2014) |
Published | 10 years, 10 months ago (Nov. 3, 2014) |
Published Online | 10 years, 10 months ago (Nov. 4, 2014) |
Published Print | 10 years, 10 months ago (Nov. 3, 2014) |
Funders
1
European Research Council
10.13039/501100000781
Region: Europe
gov (National government)
Labels
1
- ERC
Awards
1
- 306719
@article{Wang_2014, title={Exciton dynamics in WSe2 bilayers}, volume={105}, ISSN={1077-3118}, url={http://dx.doi.org/10.1063/1.4900945}, DOI={10.1063/1.4900945}, number={18}, journal={Applied Physics Letters}, publisher={AIP Publishing}, author={Wang, G. and Marie, X. and Bouet, L. and Vidal, M. and Balocchi, A. and Amand, T. and Lagarde, D. and Urbaszek, B.}, year={2014}, month=nov }