DOI: 10.1063/1.480240. Three pulse photon echo studies of nondipolar solvation: Comparison with a viscoelastic model

Three pulse photon echo studies of nondipolar solvation: Comparison with a viscoelastic model

10.1063/1.480240

Crossref journal-article

AIP Publishing

The Journal of Chemical Physics (317)

Abstract

Three pulse stimulated photon echo peak shift (3PEPS) measurements were used to probe the solvation of a quadrupolar solute in three room temperature nondipolar solvents; benzene, CCl4, and CS2, and the results were compared with those for two polar solvents, methanol and acetonitrile, and one weakly polar solvent, toluene. Our data reveal three distinct solvent dynamical time scales; a sub-100 fs ultrafast component attributed to inertial motions, a slow (∼2–3 ps) component attributed to structural relaxation, and an intermediate time scale (∼600 fs) of uncertain origin. The six solvents were chosen to reflect a range of possible interactions, but exhibit similar dynamics, suggesting that similar mechanisms may be at work or that different mechanisms may exist, but occur on similar time scales. A viscoelastic continuum solvation model proposed to describe nonpolar solvation [J. Phys. Chem. A 102, 17 (1998)] was used for a preliminary analysis of our data.

Bibliography

Larsen, D. S., Ohta, K., & Fleming, G. R. (1999). Three pulse photon echo studies of nondipolar solvation: Comparison with a viscoelastic model. The Journal of Chemical Physics, 111(19), 8970â8979.

Authors 3

Delmar S. Larsen (first)
Kaoru Ohta (additional)
Graham R. Fleming (additional)

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Dates

Type	When
Created	23 years, 1 month ago (July 26, 2002, 8:17 a.m.)
Deposited	1 year, 6 months ago (Feb. 10, 2024, 10:20 a.m.)
Indexed	1 month, 3 weeks ago (July 4, 2025, 9:24 a.m.)
Issued	25 years, 9 months ago (Nov. 15, 1999)
Published	25 years, 9 months ago (Nov. 15, 1999)
Published Print	25 years, 9 months ago (Nov. 15, 1999)

Funders 0

None

BibTeX

@article{Larsen_1999, title={Three pulse photon echo studies of nondipolar solvation: Comparison with a viscoelastic model}, volume={111}, ISSN={1089-7690}, url={http://dx.doi.org/10.1063/1.480240}, DOI={10.1063/1.480240}, number={19}, journal={The Journal of Chemical Physics}, publisher={AIP Publishing}, author={Larsen, Delmar S. and Ohta, Kaoru and Fleming, Graham R.}, year={1999}, month=nov, pages={8970–8979} }

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