DOI: 10.1063/1.476212. Exciton-migration and three-pulse femtosecond optical spectroscopies of photosynthetic antenna complexes

Exciton-migration and three-pulse femtosecond optical spectroscopies of photosynthetic antenna complexes

10.1063/1.476212

Crossref journal-article

AIP Publishing

The Journal of Chemical Physics (317)

Abstract

A theory for four-wave-mixing signals from molecular aggregates, which includes effects of two-exciton states, static disorder, and coupling to a phonon bath with an arbitrary spectral density, is developed. The third-order polarization is rigorously partitioned into a coherent and a sequential contribution. The latter is given by a sum of an exciton-hopping and a ground state (bleaching) terms, both expressed using the doorway-window representation. Applications are made to photon-echo and pump-probe spectroscopies of the B850 system of the LH2 antenna in purple bacteria.

Bibliography

Zhang, W. M., Meier, T., Chernyak, V., & Mukamel, S. (1998). Exciton-migration and three-pulse femtosecond optical spectroscopies of photosynthetic antenna complexes. The Journal of Chemical Physics, 108(18), 7763â7774.

Authors 4

Wei Min Zhang (first)
Torsten Meier (additional)
Vladimir Chernyak (additional)
Shaul Mukamel (additional)

References 44 Referenced 382

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Dates

Type	When
Created	23 years ago (July 26, 2002, 9:59 a.m.)
Deposited	1 year, 6 months ago (Feb. 5, 2024, 4:35 p.m.)
Indexed	2 weeks, 4 days ago (Aug. 6, 2025, 8:41 a.m.)
Issued	27 years, 3 months ago (May 8, 1998)
Published	27 years, 3 months ago (May 8, 1998)
Published Print	27 years, 3 months ago (May 8, 1998)

Funders 0

None

BibTeX

@article{Zhang_1998, title={Exciton-migration and three-pulse femtosecond optical spectroscopies of photosynthetic antenna complexes}, volume={108}, ISSN={1089-7690}, url={http://dx.doi.org/10.1063/1.476212}, DOI={10.1063/1.476212}, number={18}, journal={The Journal of Chemical Physics}, publisher={AIP Publishing}, author={Zhang, Wei Min and Meier, Torsten and Chernyak, Vladimir and Mukamel, Shaul}, year={1998}, month=may, pages={7763–7774} }

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