DOI: 10.1063/1.469415. Photoelectron spectroscopy of the solvated anion clusters O−(Ar)<i>n</i>=1

Photoelectron spectroscopy of the solvated anion clusters O−(Ar)n=1–26,34: Energetics and structure

10.1063/1.469415

Crossref journal-article

AIP Publishing

The Journal of Chemical Physics (317)

Abstract

Negative ion photoelectron spectra of the solvated anion clusters O−(Ar)n=1–26,34 have been recorded. Vertical detachment energies obtained from the cluster anion spectra were used to determine total as well as stepwise stabilization energies. An examination of these energetic values as a function of cluster size demonstrates that the first solvation shell closes at n=12. Furthermore, magic numbers in the energetic data and in the mass spectrum suggest O−(Ar)n clusters of sizes n=12–34 are structurally very similar to homogeneous rare gas clusters and follow a polyicosahedral packing pattern, implying O−(Ar)12 has an icosahedral structure and O−(Ar)18 has a double icosahedral structure. The solvated cluster anion photoelectron data were also analyzed using a generalized cluster size equation, which relates the cluster anion data to bulk parameters. The data for O−(Ar)n≥12 is well represented by the theoretical prediction and was therefore used to estimate several bulk parameters, including the photoemission threshold, the photoconductivity threshold, and the bulk solvation energy.

Bibliography

Arnold, S. T., Hendricks, J. H., & Bowen, K. H. (1995). Photoelectron spectroscopy of the solvated anion clusters Oâ(Ar)n=1â26,34: Energetics and structure. The Journal of Chemical Physics, 102(1), 39â47.

Authors 3

Susan T. Arnold (first)
Jay H. Hendricks (additional)
Kit H. Bowen (additional)

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Dates

Type	When
Created	23 years, 1 month ago (July 26, 2002, 8:32 a.m.)
Deposited	1 year, 6 months ago (Feb. 10, 2024, 4:03 p.m.)
Indexed	1 month, 4 weeks ago (July 3, 2025, 3:32 a.m.)
Issued	30 years, 8 months ago (Jan. 1, 1995)
Published	30 years, 8 months ago (Jan. 1, 1995)
Published Print	30 years, 8 months ago (Jan. 1, 1995)

Funders 0

None

BibTeX

@article{Arnold_1995, title={Photoelectron spectroscopy of the solvated anion clusters O−(Ar)n=1–26,34: Energetics and structure}, volume={102}, ISSN={1089-7690}, url={http://dx.doi.org/10.1063/1.469415}, DOI={10.1063/1.469415}, number={1}, journal={The Journal of Chemical Physics}, publisher={AIP Publishing}, author={Arnold, Susan T. and Hendricks, Jay H. and Bowen, Kit H.}, year={1995}, month=jan, pages={39–47} }

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