DOI: 10.1063/1.465268. Correlation effects on Raman scattering from low-energy vibrational modes in glasses. II. Experimental results

Correlation effects on Raman scattering from low-energy vibrational modes in glasses. II. Experimental results

10.1063/1.465268

Crossref journal-article

AIP Publishing

The Journal of Chemical Physics (317)

Abstract

New experimental results of low-frequency Raman scattering from different glasses are presented. They are compared to the vibration density of states obtained from inelastic neutron scattering to deduce the light-vibration coupling coefficient C(ω) as a function of the vibration frequency. It was found that C(ω)∝ω2 at very low frequency ω&lt;20 cm−1 in inorganic glasses (SiO2,B2O3) and that C(ω)∝ω at low frequency in polymer glasses and in inorganic glasses for ω≳20 cm−1. Our experimental results for glasses are interpreted by assuming no correlation at very low-frequency and only radial correlation at low-frequency. A full correlation would exist in silica-aerogels in which the effect of random fluctuations would be negligible.

Bibliography

Achibat, T., Boukenter, A., & Duval, E. (1993). Correlation effects on Raman scattering from low-energy vibrational modes in glasses. II. Experimental results. The Journal of Chemical Physics, 99(3), 2046â2051.

Authors 3

T. Achibat (first)
A. Boukenter (additional)
E. Duval (additional)

References 36 Referenced 91

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Dates

Type	When
Created	23 years, 1 month ago (July 26, 2002, 8:28 a.m.)
Deposited	1 year, 6 months ago (Feb. 10, 2024, 5:44 p.m.)
Indexed	1 year, 1 month ago (July 29, 2024, 1:09 p.m.)
Issued	32 years, 1 month ago (Aug. 1, 1993)
Published	32 years, 1 month ago (Aug. 1, 1993)
Published Print	32 years, 1 month ago (Aug. 1, 1993)

Funders 0

None

BibTeX

@article{Achibat_1993, title={Correlation effects on Raman scattering from low-energy vibrational modes in glasses. II. Experimental results}, volume={99}, ISSN={1089-7690}, url={http://dx.doi.org/10.1063/1.465268}, DOI={10.1063/1.465268}, number={3}, journal={The Journal of Chemical Physics}, publisher={AIP Publishing}, author={Achibat, T. and Boukenter, A. and Duval, E.}, year={1993}, month=aug, pages={2046–2051} }

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