DOI: 10.1063/1.463629. Periodic perturbations of the oscillatory CO oxidation on Pt(110): Model calculations

Periodic perturbations of the oscillatory CO oxidation on Pt(110): Model calculations

10.1063/1.463629

Crossref journal-article

AIP Publishing

The Journal of Chemical Physics (317)

Abstract

The periodically perturbed oscillations in the isothermal CO oxidation on a Pt(110) surface at low pressure were modeled using the recently developed reconstruction model of kinetic oscillations, in which the usual Langmuir–Hinshelwood mechanism is coupled with the CO-driven 1×2⇄1×1 phase transition of the surface. The experimental findings (entrainment bands, quasiperiodicity, critical slowing down) could be well reproduced with this model. The calculations revealed a complicated bifurcation fine structure of the Arnol’d tongues. While the skeleton structure turned out to be the same as in other studies, some additional features were found, and several details (mainly in the p/2 tongues) were different from forced systems examined previously. A co-dimension-3 bifurcation (in which a second-order resonance coincides with a degenerate period doubling) is discussed in this context.

Bibliography

Krischer, K., Eiswirth, M., & Ertl, G. (1992). Periodic perturbations of the oscillatory CO oxidation on Pt(110): Model calculations. The Journal of Chemical Physics, 97(1), 307â319.

Authors 3

K. Krischer (first)
M. Eiswirth (additional)
G. Ertl (additional)

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Dates

Type	When
Created	23 years, 1 month ago (July 26, 2002, 8:22 a.m.)
Deposited	1 year, 6 months ago (Feb. 10, 2024, 9:40 a.m.)
Indexed	1 year, 6 months ago (Feb. 10, 2024, 6:02 p.m.)
Issued	33 years, 2 months ago (July 1, 1992)
Published	33 years, 2 months ago (July 1, 1992)
Published Print	33 years, 2 months ago (July 1, 1992)

Funders 0

None

BibTeX

@article{Krischer_1992, title={Periodic perturbations of the oscillatory CO oxidation on Pt(110): Model calculations}, volume={97}, ISSN={1089-7690}, url={http://dx.doi.org/10.1063/1.463629}, DOI={10.1063/1.463629}, number={1}, journal={The Journal of Chemical Physics}, publisher={AIP Publishing}, author={Krischer, K. and Eiswirth, M. and Ertl, G.}, year={1992}, month=jul, pages={307–319} }

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