DOI: 10.1063/1.460467. Creation and dynamics of molecular states prepared with coherent vs partially coherent pulsed light

Creation and dynamics of molecular states prepared with coherent vs partially coherent pulsed light

10.1063/1.460467

Crossref journal-article

AIP Publishing

The Journal of Chemical Physics (317)

Abstract

The mixed state of an isolated molecule, which results from one-photon absorption using a pulsed laser of arbitrary coherence, is obtained using a simple model for a partially coherent laser source. The relative effect of the pulse time τ, source coherence time τcoh, and field correlation time τc on the prepared state and on its subsequent molecular dynamics are described. Numerical computations on several properties are provided and support obtained for the analytical result showing that under certain circumstances the falloff of the survival probability of the created molecular state depends primarily on the pulse time τ.

Bibliography

Jiang, X.-P., & Brumer, P. (1991). Creation and dynamics of molecular states prepared with coherent vs partially coherent pulsed light. The Journal of Chemical Physics, 94(9), 5833â5843.

Authors 2

Xue-Pei Jiang (first)
Paul Brumer (additional)

References 35 Referenced 82

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{'key': '2024021011050171500_r8'}
{'key': '2024021011050171500_r8a'}
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Dates

Type	When
Created	23 years, 1 month ago (July 26, 2002, 8:20 a.m.)
Deposited	1 year, 6 months ago (Feb. 10, 2024, 7:51 a.m.)
Indexed	2 months ago (July 2, 2025, 11:39 a.m.)
Issued	34 years, 4 months ago (May 1, 1991)
Published	34 years, 4 months ago (May 1, 1991)
Published Print	34 years, 4 months ago (May 1, 1991)

Funders 0

None

BibTeX

@article{Jiang_1991, title={Creation and dynamics of molecular states prepared with coherent vs partially coherent pulsed light}, volume={94}, ISSN={1089-7690}, url={http://dx.doi.org/10.1063/1.460467}, DOI={10.1063/1.460467}, number={9}, journal={The Journal of Chemical Physics}, publisher={AIP Publishing}, author={Jiang, Xue-Pei and Brumer, Paul}, year={1991}, month=may, pages={5833–5843} }

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