DOI: 10.1063/1.451268. Time resolved study of the Fermi component Ω−(Ag) in solid CO2 at <i>T</i>≂5 K

Time resolved study of the Fermi component Ω−(Ag) in solid CO2 at T≂5 K

10.1063/1.451268

Crossref journal-article

AIP Publishing

The Journal of Chemical Physics (317)

Abstract

We have investigated the vibrational coherence relaxation for the long-living Ω−(Ag) hybrid bound state of the Fermi diad ω1:2ω2 in natural crystalline CO2 at T≂5 K by means of time resolved nanosecond CARS spectroscopy. The decay profile was found to be slower than exponential and fitting reasonably well to an exp{−(t/τ)1/2} time dependence with τ=2.3±0.2 ns. Our results are discussed in terms of weak diagonal structural disorder upon the vibrational relaxation of exciton states located near the band edges.

Bibliography

Ouillon, R., & Ranson, P. (1986). Time resolved study of the Fermi component Î©â(Ag) in solid CO2 at Tâ5 K. The Journal of Chemical Physics, 85(3), 1295â1298.

Authors 2

R. Ouillon (first)
P. Ranson (additional)

References 24 Referenced 12

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{'key': '2024021003304651500_r5'}
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Dates

Type	When
Created	23 years, 1 month ago (July 26, 2002, 9:02 a.m.)
Deposited	1 year, 6 months ago (Feb. 9, 2024, 11:48 p.m.)
Indexed	1 year, 6 months ago (Feb. 10, 2024, 8:45 a.m.)
Issued	39 years, 1 month ago (Aug. 1, 1986)
Published	39 years, 1 month ago (Aug. 1, 1986)
Published Print	39 years, 1 month ago (Aug. 1, 1986)

Funders 0

None

BibTeX

@article{Ouillon_1986, title={Time resolved study of the Fermi component Ω−(Ag) in solid CO2 at T≂5 K}, volume={85}, ISSN={1089-7690}, url={http://dx.doi.org/10.1063/1.451268}, DOI={10.1063/1.451268}, number={3}, journal={The Journal of Chemical Physics}, publisher={AIP Publishing}, author={Ouillon, R. and Ranson, P.}, year={1986}, month=aug, pages={1295–1298} }

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