DOI: 10.1063/1.451242. Effects of periodic perturbations on the oscillatory combustion of acetaldehyde

Effects of periodic perturbations on the oscillatory combustion of acetaldehyde

10.1063/1.451242

Crossref journal-article

AIP Publishing

The Journal of Chemical Physics (317)

Abstract

Periodic perturbations are applied to the input rates of acetaldehyde and oxygen, one at a time, in the combustion of acetaldehyde in a CSTR. We measure periodic responses in five entrainment bands as we vary the frequency and amplitude of the external periodic perturbation. Outside of entrainment bands we find quasiperiodic responses. Next-phase maps of the experimental results are constructed in real time and used in the observation and interpretation of entrainment and quasiperiodic behavior. Within the fundamental entrainment band, we measure critical slowing down and enhancement of the response amplitude. As the bath temperature is increased, so that the oscillatory system approaches a Hopf bifurcation, we observe an increase in the amplitude enhancement. The predictions of a five-variable thermokinetic model agree with the experimental results.

Bibliography

Pugh, S. A., Schell, M., & Ross, J. (1986). Effects of periodic perturbations on the oscillatory combustion of acetaldehyde. The Journal of Chemical Physics, 85(2), 868â878.

Authors 3

Spencer A. Pugh (first)
Mark Schell (additional)
John Ross (additional)

References 35 Referenced 33

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Dates

Type	When
Created	23 years, 1 month ago (July 26, 2002, 9:02 a.m.)
Deposited	1 year, 6 months ago (Feb. 9, 2024, 11:44 p.m.)
Indexed	1 year, 6 months ago (Feb. 10, 2024, 10:25 a.m.)
Issued	39 years, 1 month ago (July 15, 1986)
Published	39 years, 1 month ago (July 15, 1986)
Published Print	39 years, 1 month ago (July 15, 1986)

Funders 0

None

BibTeX

@article{Pugh_1986, title={Effects of periodic perturbations on the oscillatory combustion of acetaldehyde}, volume={85}, ISSN={1089-7690}, url={http://dx.doi.org/10.1063/1.451242}, DOI={10.1063/1.451242}, number={2}, journal={The Journal of Chemical Physics}, publisher={AIP Publishing}, author={Pugh, Spencer A. and Schell, Mark and Ross, John}, year={1986}, month=jul, pages={868–878} }

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