DOI: 10.1063/1.444128. Intermolecular transfer and quenching of electronic excitation energy in fluid solutions: Interpretation of experimental data with a diffusion model including distance dependent interaction

Intermolecular transfer and quenching of electronic excitation energy in fluid solutions: Interpretation of experimental data with a diffusion model including distance dependent interaction

10.1063/1.444128

Crossref journal-article

AIP Publishing

The Journal of Chemical Physics (317)

Abstract

The efficiency for the transfer of the electronic excitation between moving molecules is analyzed by means of a diffusion equation taking into account long and/or short range interactions. The analysis of experimental data concerning donor–acceptor systems with large Förster radius in viscous and fluid solvents demonstrates that (i) in the low diffusion regime, energy transfer takes place by the resonant dipole–dipole mechanism; (ii) for high diffusivities, the efficient interaction is not that of the dipole–dipole type, and exchange interactions are responsible for the energy transfer. Experimental efficiencies of fluorescence quenching by an intermolecular charge transfer mechanism are interpreted in view of the diffusion model including a specular boundary condition and an exponential sink term of short range. It is apparent that the diffusion tends to increase the effective quenching rate for strongly coupled interacting donor–inhibitor species to a greater extent than for weakly coupled ones. Effective reaction radii larger than those predicted by diffusion-controlled reactions are interpreted.

Bibliography

Heisel, F., & Miehe, J. A. (1982). Intermolecular transfer and quenching of electronic excitation energy in fluid solutions: Interpretation of experimental data with a diffusion model including distance dependent interaction. The Journal of Chemical Physics, 77(5), 2558â2569.

Authors 2

F. Heisel (first)
J. A. Miehe (additional)

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Dates

Type	When
Created	22 years, 5 months ago (Feb. 28, 2003, 11:32 a.m.)
Deposited	1 year, 6 months ago (Feb. 9, 2024, 7:21 p.m.)
Indexed	1 year, 6 months ago (Feb. 10, 2024, 10:21 a.m.)
Issued	42 years, 11 months ago (Sept. 1, 1982)
Published	42 years, 11 months ago (Sept. 1, 1982)
Published Print	42 years, 11 months ago (Sept. 1, 1982)

Funders 0

None

BibTeX

@article{Heisel_1982, title={Intermolecular transfer and quenching of electronic excitation energy in fluid solutions: Interpretation of experimental data with a diffusion model including distance dependent interaction}, volume={77}, ISSN={1089-7690}, url={http://dx.doi.org/10.1063/1.444128}, DOI={10.1063/1.444128}, number={5}, journal={The Journal of Chemical Physics}, publisher={AIP Publishing}, author={Heisel, F. and Miehe, J. A.}, year={1982}, month=sep, pages={2558–2569} }

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