DOI: 10.1063/1.441006. Vibrational product states from reactions of CN− with the hydrogen halides and hydrogen atoms

Vibrational product states from reactions of CN− with the hydrogen halides and hydrogen atoms

10.1063/1.441006

Crossref journal-article

AIP Publishing

The Journal of Chemical Physics (317)

Abstract

Infrared chemiluminescence is observed from the C–H stretch manifold ν3 of HCN formed in the gas phase ion–molecule reactions: CN−+HX→HCN(v3)+X−, with (X = Cl, Br, I), and for CN−+H→HCN(v3)+e−. Qualitative information is also obtained for excitation in the bending mode. In each case some excitation is observed in the highest level allowed by energy conservation. Comparison with similar studies of the reactions Cl−+HX shows that the stretching mode of the newly formed bond is less efficiently populated in the HCN case. Emission is observed from CNH (hydroisocyanic acid) formed in the reaction CN−+HI→CNH(v)+I−.

Bibliography

Maricq, M. M., Smith, M. A., Simpson, C. J. S. M., & Ellison, G. B. (1981). Vibrational product states from reactions of CNâ with the hydrogen halides and hydrogen atoms. The Journal of Chemical Physics, 74(11), 6154â6170.

Authors 4

M. Matti Maricq (first)
Mark A. Smith (additional)
C. J. S. M. Simpson (additional)
G. Barney Ellison (additional)

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Dates

Type	When
Created	22 years, 5 months ago (Feb. 28, 2003, 10:46 a.m.)
Deposited	1 year, 6 months ago (Feb. 9, 2024, 5:32 p.m.)
Indexed	1 year, 6 months ago (Feb. 10, 2024, 10:25 a.m.)
Issued	44 years, 2 months ago (June 1, 1981)
Published	44 years, 2 months ago (June 1, 1981)
Published Print	44 years, 2 months ago (June 1, 1981)

Funders 0

None

BibTeX

@article{Maricq_1981, title={Vibrational product states from reactions of CN− with the hydrogen halides and hydrogen atoms}, volume={74}, ISSN={1089-7690}, url={http://dx.doi.org/10.1063/1.441006}, DOI={10.1063/1.441006}, number={11}, journal={The Journal of Chemical Physics}, publisher={AIP Publishing}, author={Maricq, M. Matti and Smith, Mark A. and Simpson, C. J. S. M. and Ellison, G. Barney}, year={1981}, month=jun, pages={6154–6170} }

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  "abstract": "<jats:p>Infrared chemiluminescence is observed from the C\u2013H stretch manifold \u03bd3 of HCN formed in the gas phase ion\u2013molecule reactions: CN\u2212+HX\u2192HCN(v3)+X\u2212, with (X = Cl, Br, I), and for CN\u2212+H\u2192HCN(v3)+e\u2212. Qualitative information is also obtained for excitation in the bending mode. In each case some excitation is observed in the highest level allowed by energy conservation. Comparison with similar studies of the reactions Cl\u2212+HX shows that the stretching mode of the newly formed bond is less efficiently populated in the HCN case. Emission is observed from CNH (hydroisocyanic acid) formed in the reaction CN\u2212+HI\u2192CNH(v)+I\u2212.</jats:p>",
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