DOI: 10.1063/1.438689. Non-Markovian theory of collisional dephasing in near resonance light scattering

Non-Markovian theory of collisional dephasing in near resonance light scattering

10.1063/1.438689

Crossref journal-article

AIP Publishing

The Journal of Chemical Physics (317)

Abstract

We present a general microscopic theory for near resonance light scattering (RLS) from collisionally perturbed atoms and molecules. The theory is based on the tetradic scattering formalism of Fano and Ben-Reuven. We perform a systematic density expansion and show that the four-time, many-body, dipole correlation functions necessary for the evaluation of the RLS cross section may be rigorously expressed (to lowest order in pressure) in terms of three single-particle, two-time, correlation functions, two of which are associated with the absorption and emission line broadening and the third is a cross correlation function. Our most general expressions are valid for an arbitrary value of the bath correlation time (relative to the broadening), and interpolate smoothly all the way from the static limit of inhomogenous broadening up to the reverse, the Markovian (homogenous) limit. The stochastic Gaussian model of Takagahara, Hanamura, and Kubo is obtained also as a special case of the present formulation.

Bibliography

Mukamel, S. (1979). Non-Markovian theory of collisional dephasing in near resonance light scattering. The Journal of Chemical Physics, 71(7), 2884â2891.

Authors 1

Shaul Mukamel (first)

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Dates

Type	When
Created	22 years, 6 months ago (Feb. 27, 2003, 4:39 p.m.)
Deposited	1 year, 6 months ago (Feb. 9, 2024, 3:36 p.m.)
Indexed	1 year, 2 months ago (June 15, 2024, 7:37 p.m.)
Issued	45 years, 11 months ago (Oct. 1, 1979)
Published	45 years, 11 months ago (Oct. 1, 1979)
Published Print	45 years, 11 months ago (Oct. 1, 1979)

Funders 0

None

BibTeX

@article{Mukamel_1979, title={Non-Markovian theory of collisional dephasing in near resonance light scattering}, volume={71}, ISSN={1089-7690}, url={http://dx.doi.org/10.1063/1.438689}, DOI={10.1063/1.438689}, number={7}, journal={The Journal of Chemical Physics}, publisher={AIP Publishing}, author={Mukamel, Shaul}, year={1979}, month=oct, pages={2884–2891} }

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