DOI: 10.1063/1.437605. Laser-stimulated migration of adsorbed atoms on solid surfaces

Laser-stimulated migration of adsorbed atoms on solid surfaces

10.1063/1.437605

Crossref journal-article

AIP Publishing

The Journal of Chemical Physics (317)

Abstract

This paper presents a unified theory of the coherent, multiple-photon excitation and laser-stimulated migration of atoms adsorbed on solid surfaces. We show that under steady-state excitation the migration of the adsorbed atom on the surface is diffusional, with diffusion constant dependent upon field intensity, surface temperature, relaxation constants, dipole moment strength, laser frequency, and the vibrational frequency of the adsorbed atom. In particular, it is shown that the rate of diffusion is proportional to the field intensity. Finally, we discuss the utility of laser-stimulated migration in the enhancement of surface chemical reactions, as well as in the analysis of surface relaxational processes.

Bibliography

Slutsky, M. S., & George, T. F. (1979). Laser-stimulated migration of adsorbed atoms on solid surfaces. The Journal of Chemical Physics, 70(3), 1231â1235.

Authors 2

M. S. Slutsky (first)
Thomas F. George (additional)

References 18 Referenced 26

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{'key': '2024020917383482500_r3'}
{'key': '2024020917383482500_r4'}
10.1016/0009-2614(78)85553-5 / Chem. Phys. Lett. (1978)
10.1063/1.434577 / J. Chem. Phys. (1977)
10.1063/1.436159 / J. Chem. Phys. (1978)
10.1016/0009-2614(76)80789-0 / Chem. Phys. Lett. (1976)
10.1063/1.433437 / J. Chem. Phys. (1976)
10.1016/0039-6028(78)90189-9 / Surf. Sci. (1978)
10.1063/1.436938 / J. Chem. Phys. (1978)
{'key': '2024020917383482500_r10'}
10.1103/PhysRevB.1.3966 / Phys. Rev. B (1970)
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Dates

Type	When
Created	22 years, 6 months ago (Feb. 27, 2003, 5:52 p.m.)
Deposited	1 year, 6 months ago (Feb. 9, 2024, 2:32 p.m.)
Indexed	1 year, 6 months ago (Feb. 9, 2024, 10:43 p.m.)
Issued	46 years, 7 months ago (Feb. 1, 1979)
Published	46 years, 7 months ago (Feb. 1, 1979)
Published Print	46 years, 7 months ago (Feb. 1, 1979)

Funders 0

None

BibTeX

@article{Slutsky_1979, title={Laser-stimulated migration of adsorbed atoms on solid surfaces}, volume={70}, ISSN={1089-7690}, url={http://dx.doi.org/10.1063/1.437605}, DOI={10.1063/1.437605}, number={3}, journal={The Journal of Chemical Physics}, publisher={AIP Publishing}, author={Slutsky, M. S. and George, Thomas F.}, year={1979}, month=feb, pages={1231–1235} }

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