DOI: 10.1063/1.3225154. Tuning electronic and magnetic properties of graphene by surface modification

Tuning electronic and magnetic properties of graphene by surface modification

10.1063/1.3225154

Crossref journal-article

AIP Publishing

Applied Physics Letters (317)

Abstract

We have demonstrated that the electronic and magnetic properties of graphene sheet can be delicately tuned by surface modification. Applying an external electric field to a fully hydrogenated graphene sheet can unload hydrogen atoms on one side, while keeping the hydrogen atoms on the other side, thus forming a half-hydrogenated graphene sheet, where the unpaired electrons in the unsaturated C sites give rise to magnetic moments, coupled through extended p-p interactions. Furthermore, the electronic structure of the resulting half-hydrogenated graphene sheet can be further tuned by introducing F atoms on the other side, making a nonmagnetic semiconductor with a direct band gap.

Bibliography

Zhou, J., Wu, M. M., Zhou, X., & Sun, Q. (2009). Tuning electronic and magnetic properties of graphene by surface modification. Applied Physics Letters, 95(10).

Authors 4

Jian Zhou (first)
Miao Miao Wu (additional)
Xiao Zhou (additional)
Qiang Sun (additional)

References 20 Referenced 205

10.1126/science.1102896 / Science (2004)
10.1103/PhysRevB.75.153401 / Phys. Rev. B (2007)
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10.1002/1521-3773(20010618)40:12<2285::AID-ANIE2285>3.0.CO;2-Y / Angew. Chem., Int. Ed. (2001)
10.1021/ja0781590 / J. Am. Chem. Soc. (2008)
10.1126/science.1111904 / Science (2005)
10.1063/1.1828595 / Appl. Phys. Lett. (2004)
10.1103/PhysRevB.63.045413 / Phys. Rev. B (2001)
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Dates

Type	When
Created	15 years, 11 months ago (Sept. 9, 2009, 6:35 p.m.)
Deposited	2 years, 1 month ago (July 2, 2023, 6:40 p.m.)
Indexed	2 weeks, 3 days ago (Aug. 6, 2025, 9:29 a.m.)
Issued	15 years, 11 months ago (Sept. 7, 2009)
Published	15 years, 11 months ago (Sept. 7, 2009)
Published Online	15 years, 11 months ago (Sept. 9, 2009)
Published Print	15 years, 11 months ago (Sept. 7, 2009)

Funders 0

None

BibTeX

@article{Zhou_2009, title={Tuning electronic and magnetic properties of graphene by surface modification}, volume={95}, ISSN={1077-3118}, url={http://dx.doi.org/10.1063/1.3225154}, DOI={10.1063/1.3225154}, number={10}, journal={Applied Physics Letters}, publisher={AIP Publishing}, author={Zhou, Jian and Wu, Miao Miao and Zhou, Xiao and Sun, Qiang}, year={2009}, month=sep }

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