DOI: 10.1063/1.2424706. Manipulating multidimensional electronic spectra of excitons by polarization pulse shaping

Manipulating multidimensional electronic spectra of excitons by polarization pulse shaping

10.1063/1.2424706

Crossref journal-article

AIP Publishing

The Journal of Chemical Physics (317)

Abstract

A simulation study demonstrates how coherent control, combined with adaptive polarization pulse shaping and a genetic algorithm, may be used to simplify femtosecond coherent nonlinear optical signals of excitons. Cross peaks are amplified and resolved, and diagonal peaks are suppressed in the heterodyne-detected two-pulse echo signal from the Soret band of a porphyrin dimer coupled to a Brownian oscillator bath. Various optimization strategies involving the spectral, temporal, and polarization profiles of the second pulse are compared.

Bibliography

Voronine, D. V., Abramavicius, D., & Mukamel, S. (2007). Manipulating multidimensional electronic spectra of excitons by polarization pulse shaping. The Journal of Chemical Physics, 126(4).

Authors 3

Dmitri V. Voronine (first)
Darius Abramavicius (additional)
Shaul Mukamel (additional)

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Dates

Type	When
Created	18 years, 7 months ago (Feb. 3, 2007, 1:30 a.m.)
Deposited	2 years, 1 month ago (July 31, 2023, 4:03 p.m.)
Indexed	1 month, 1 week ago (July 30, 2025, 6:48 a.m.)
Issued	18 years, 7 months ago (Jan. 28, 2007)
Published	18 years, 7 months ago (Jan. 28, 2007)
Published Online	18 years, 7 months ago (Jan. 31, 2007)
Published Print	18 years, 7 months ago (Jan. 28, 2007)

Funders 0

None

BibTeX

@article{Voronine_2007, title={Manipulating multidimensional electronic spectra of excitons by polarization pulse shaping}, volume={126}, ISSN={1089-7690}, url={http://dx.doi.org/10.1063/1.2424706}, DOI={10.1063/1.2424706}, number={4}, journal={The Journal of Chemical Physics}, publisher={AIP Publishing}, author={Voronine, Dmitri V. and Abramavicius, Darius and Mukamel, Shaul}, year={2007}, month=jan }

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