Abstract
A thermodynamic model is presented that describes the polarization and the dielectric response of ferroelectric-paraelectric bilayers and multilayers. It is shown that a strong electrostatic coupling between the layers results in the suppression of ferroelectricity at a critical paraelectric layer thickness. The bilayer is expected to have a gigantic dielectric response similar to the dielectric anomaly near Curie–Weiss temperature in homogeneous ferroelectrics at this critical thickness. A numerical analysis is carried out for a pseudomorphic (001) BaTiO3∕SrTiO3 heteroepitaxial bilayer on (001) SrTiO3 and a stress-free BaTiO3∕SrTiO3 bilayer. Complete polarization suppression and a dielectric peak are predicted to occur at approximately 66% and 14% of SrTiO3 in these two systems, respectively.
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Dates
Type | When |
---|---|
Created | 20 years ago (Aug. 19, 2005, 6 p.m.) |
Deposited | 2 years, 2 months ago (June 30, 2023, 10:55 p.m.) |
Indexed | 1 month ago (July 30, 2025, 6:46 a.m.) |
Issued | 20 years ago (Aug. 22, 2005) |
Published | 20 years ago (Aug. 22, 2005) |
Published Online | 20 years ago (Aug. 22, 2005) |
Published Print | 20 years ago (Aug. 29, 2005) |
@article{Roytburd_2005, title={Dielectric anomaly due to electrostatic coupling in ferroelectric-paraelectric bilayers and multilayers}, volume={87}, ISSN={1077-3118}, url={http://dx.doi.org/10.1063/1.2032601}, DOI={10.1063/1.2032601}, number={9}, journal={Applied Physics Letters}, publisher={AIP Publishing}, author={Roytburd, A. L. and Zhong, S. and Alpay, S. P.}, year={2005}, month=aug }