Abstract
The depolarized light mixing (DLM) system is presented as a useful device in light beating spectroscopy for the observation of molecular rotation, deformation, and reaction which accompany an anisotropic change of polarizability. The system has the following merits: (1) Doppler broadening does not appear because it observes forward scattering; (2) only the line shape coming from a pure anisotropic polarizability change is obtained; (3) it can work automatically as an optical heterodyne system with the stray light from the second polarizer serving as a local oscillator light; (4) there is no difficulty in matching the wavefronts of the scattered light and local oscillator beam; and (5) the scattering volume can be made large without diminishing the efficiency of light beating. These characteristics are described through the numerical evaluation of beating efficiency and signal-to-noise ratio.
References
6
Referenced
14
{'key': '2024020612343623000_r1'}
10.1063/1.1670794
/ J. Chem. Phys. (1969){'key': '2024020612343623000_r3', 'first-page': '892', 'volume': '37', 'year': '1968', 'journal-title': 'J. Appl. Phys. Japan'}
/ J. Appl. Phys. Japan (1968)10.1364/JOSA.51.000253
/ J. Opt. Soc. Amer. (1961){'key': '2024020612343623000_r5', 'first-page': '1604', 'volume': '40', 'year': '1969', 'journal-title': 'J. Chem. Phys.'}
/ J. Chem. Phys. (1969)10.1063/1.1669427
/ J. Chem. Phys. (1968)
Dates
Type | When |
---|---|
Created | 21 years, 6 months ago (Feb. 10, 2004, 4:49 p.m.) |
Deposited | 1 year, 6 months ago (Feb. 6, 2024, 8:14 a.m.) |
Indexed | 1 year, 6 months ago (Feb. 9, 2024, 1:02 p.m.) |
Issued | 55 years, 2 months ago (June 1, 1970) |
Published | 55 years, 2 months ago (June 1, 1970) |
Published Print | 55 years, 2 months ago (June 1, 1970) |
@article{Wada_1970, title={Depolarized Light Mixing for Light Beating Spectroscopy}, volume={41}, ISSN={1089-7623}, url={http://dx.doi.org/10.1063/1.1684661}, DOI={10.1063/1.1684661}, number={6}, journal={Review of Scientific Instruments}, publisher={AIP Publishing}, author={Wada, Akiyoshi and Soda, Kunitsugu and Tanaka, Toyoichi and Suda, Nobuhiro}, year={1970}, month=jun, pages={845–853} }