DOI: 10.1063/1.1666984. Frequency-stabilized single-mode cavity ring-down apparatus for high-resolution absorption spectroscopy

Frequency-stabilized single-mode cavity ring-down apparatus for high-resolution absorption spectroscopy

10.1063/1.1666984

Crossref journal-article

AIP Publishing

Review of Scientific Instruments (317)

Abstract

We present a cavity ring-down spectroscopy apparatus suitable for high-resolution absorption spectroscopy. The central feature of the spectrometer is a ring-down cavity whose comb of eigenfrequencies is actively stabilized with respect to a tuneable, frequency-stabilized reference laser. By using dichroic ring-down cavity mirrors that are designed to have relatively high losses and low losses at the respective wavelengths of the reference laser and probe laser, the cavity stabilization dynamics are decoupled from frequency jitter of the probe laser. We use the cavity eigenfrequencies as markers in spectral scans and achieve a frequency resolution of ≈1 MHz. Five rovibrational transitions in the (2,0,1) vibrational band of water vapor near 0.935 μm are probed with a continuous-wave external-cavity diode laser, and their line strengths are determined and compared to literature values. Collisional narrowing effects and pressure shifting are observed, illustrating the applicability of the method for quantitative line shape studies of weakly absorbing systems.

Bibliography

Hodges, J. T., Layer, H. P., Miller, W. W., & Scace, G. E. (2004). Frequency-stabilized single-mode cavity ring-down apparatus for high-resolution absorption spectroscopy. Review of Scientific Instruments, 75(4), 849â863.

Authors 4

Joseph T. Hodges (first)
Howard P. Layer (additional)
William W. Miller (additional)
Gregory E. Scace (additional)

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Dates

Type	When
Created	21 years, 5 months ago (March 20, 2004, 4:30 a.m.)
Deposited	1 year, 6 months ago (Feb. 6, 2024, 8:27 a.m.)
Indexed	3 weeks ago (Aug. 6, 2025, 9:22 a.m.)
Issued	21 years, 4 months ago (April 1, 2004)
Published	21 years, 4 months ago (April 1, 2004)
Published Print	21 years, 4 months ago (April 1, 2004)

Funders 0

None

BibTeX

@article{Hodges_2004, title={Frequency-stabilized single-mode cavity ring-down apparatus for high-resolution absorption spectroscopy}, volume={75}, ISSN={1089-7623}, url={http://dx.doi.org/10.1063/1.1666984}, DOI={10.1063/1.1666984}, number={4}, journal={Review of Scientific Instruments}, publisher={AIP Publishing}, author={Hodges, Joseph T. and Layer, Howard P. and Miller, William W. and Scace, Gregory E.}, year={2004}, month=apr, pages={849–863} }

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