Abstract
A high pressure photoemission system is described that combines differential pumping with an electrostatic lens system. This approach allows optimized differential pumping without loss of signal, thereby increasing the high-pressure performance by at least 2 orders of magnitude compared to passive differential pumping systems. A general analysis of aperture-based high-pressure photoemission is presented, followed by a description of the prototype system which has operated at pressures up to 7 mbar on a synchrotron beamline. Using this approach, photoemission experiments should be possible up to 100 mbar. Example data are presented for dielectric samples in gas atmospheres, for a copper catalyst under reaction conditions, and for liquid water in equilibrium with its vapor.
References
25
Referenced
460
{'key': '2024021013515699500_r1'}
{'key': '2024021013515699500_r2'}
{'key': '2024021013515699500_r3'}
10.1016/0368-2048(95)02545-6
/ J. Electron Spectrosc. Relat. Phenom. (1995){'key': '2024021013515699500_r5'}
10.1016/0368-2048(73)80023-4
/ J. Electron Spectrosc. Relat. Phenom. (1973)10.1016/0368-2048(75)85006-7
/ J. Electron Spectrosc. Relat. Phenom. (1975)10.1016/0368-2048(81)80007-2
/ J. Electron Spectrosc. Relat. Phenom. (1981)10.1016/0039-6028(79)90544-2
/ Surf. Sci. (1979)10.1002/sia.740150403
/ Surf. Interface Anal. (1990)10.1116/1.1374618
/ J. Vac. Sci. Technol. A (2001){'key': '2024021013515699500_r10'}
{'key': '2024021013515699500_r11', 'first-page': 'L227', 'volume': '14', 'year': '2002', 'journal-title': 'J. Phys.: Condens. Matter'}
/ J. Phys.: Condens. Matter (2002){'key': '2024021013515699500_r12'}
{'key': '2024021013515699500_r13'}
{'key': '2024021013515699500_r14'}
{'key': '2024021013515699500_r15'}
{'key': '2024021013515699500_r16'}
{'key': '2024021013515699500_r17'}
{'key': '2024021013515699500_r18'}
{'key': '2024021013515699500_r19'}
{'key': '2024021013515699500_r20'}
{'key': '2024021013515699500_r21', 'first-page': '11322', 'volume': '38', 'year': '1998', 'journal-title': 'Phys. Rev. B'}
/ Phys. Rev. B (1998){'key': '2024021013515699500_r22', 'first-page': '11', 'year': '1995'}
(1995){'key': '2024021013515699500_r23', 'first-page': 'L213', 'volume': '14', 'year': '2002', 'journal-title': 'J. Phys.: Condens. Matter'}
/ J. Phys.: Condens. Matter (2002)
Dates
Type | When |
---|---|
Created | 22 years, 9 months ago (Oct. 31, 2002, 1:22 p.m.) |
Deposited | 1 year, 6 months ago (Feb. 10, 2024, 10:18 a.m.) |
Indexed | 11 hours, 57 minutes ago (Aug. 28, 2025, 8:48 a.m.) |
Issued | 22 years, 9 months ago (Nov. 1, 2002) |
Published | 22 years, 9 months ago (Nov. 1, 2002) |
Published Print | 22 years, 9 months ago (Nov. 1, 2002) |
@article{Ogletree_2002, title={A differentially pumped electrostatic lens system for photoemission studies in the millibar range}, volume={73}, ISSN={1089-7623}, url={http://dx.doi.org/10.1063/1.1512336}, DOI={10.1063/1.1512336}, number={11}, journal={Review of Scientific Instruments}, publisher={AIP Publishing}, author={Ogletree, D. Frank and Bluhm, Hendrik and Lebedev, Gennadi and Fadley, Charles S. and Hussain, Zahid and Salmeron, Miquel}, year={2002}, month=nov, pages={3872–3877} }