Abstract
We have studied ultraviolet photoluminescence from high-purity zinc-oxide powder over a wide temperature range (2–293 K). At low temperatures, the spontaneous emission is due to radiative recombination of excitons bound to donors and acceptors. At high temperature (>90 K), it mainly consists of recombination of free excitons, with exciton–exciton collision-induced recombination dominating the spectrum at higher pumping intensities. Emission from the exciton–exciton collision process shows clear stimulated-emission behavior. At sufficiently high pumping intensity, the stimulated emission band shifts abruptly to a longer wavelength due to the formation of an electron–hole plasma. Sharp emission peaks are observed in the stimulated emission bands. The possible origins of these sharp peaks are discussed.
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Dates
Type | When |
---|---|
Created | 23 years, 1 month ago (July 26, 2002, 8:41 a.m.) |
Deposited | 1 year, 6 months ago (Feb. 3, 2024, 1:55 p.m.) |
Indexed | 1 year, 1 month ago (July 5, 2024, 5:17 p.m.) |
Issued | 24 years, 10 months ago (Oct. 9, 2000) |
Published | 24 years, 10 months ago (Oct. 9, 2000) |
Published Print | 24 years, 10 months ago (Oct. 9, 2000) |
@article{Sun_2000, title={Excitonic gain and stimulated ultraviolet emission in nanocrystalline zinc-oxide powder}, volume={77}, ISSN={1077-3118}, url={http://dx.doi.org/10.1063/1.1316069}, DOI={10.1063/1.1316069}, number={15}, journal={Applied Physics Letters}, publisher={AIP Publishing}, author={Sun, Y. and Ketterson, J. B. and Wong, G. K. L.}, year={2000}, month=oct, pages={2322–2324} }