DOI: 10.1063/1.1286035. Relaxation in glassforming liquids and amorphous solids

Relaxation in glassforming liquids and amorphous solids

10.1063/1.1286035

Crossref journal-article

AIP Publishing

Journal of Applied Physics (317)

Abstract

The field of viscous liquid and glassy solid dynamics is reviewed by a process of posing the key questions that need to be answered, and then providing the best answers available to the authors and their advisors at this time. The subject is divided into four parts, three of them dealing with behavior in different domains of temperature with respect to the glass transition temperature, Tg, and a fourth dealing with “short time processes.” The first part tackles the high temperature regime T&gt;Tg, in which the system is ergodic and the evolution of the viscous liquid toward the condition at Tg is in focus. The second part deals with the regime T∼Tg, where the system is nonergodic except for very long annealing times, hence has time-dependent properties (aging and annealing). The third part discusses behavior when the system is completely frozen with respect to the primary relaxation process but in which secondary processes, particularly those responsible for “superionic” conductivity, and dopart mobility in amorphous silicon, remain active. In the fourth part we focus on the behavior of the system at the crossover between the low frequency vibrational components of the molecular motion and its high frequency relaxational components, paying particular attention to very recent developments in the short time dielectric response and the high Q mechanical response.

Bibliography

Angell, C. A., Ngai, K. L., McKenna, G. B., McMillan, P. F., & Martin, S. W. (2000). Relaxation in glassforming liquids and amorphous solids. Journal of Applied Physics, 88(6), 3113â3157.

Authors 5

C. A. Angell (first)
K. L. Ngai (additional)
G. B. McKenna (additional)
P. F. McMillan (additional)
S. W. Martin (additional)

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Dates

Type	When
Created	23 years, 1 month ago (July 26, 2002, 9:57 a.m.)
Deposited	1 year, 6 months ago (Feb. 5, 2024, 11:02 p.m.)
Indexed	2 days, 10 hours ago (Sept. 3, 2025, 7:06 a.m.)
Issued	24 years, 11 months ago (Sept. 15, 2000)
Published	24 years, 11 months ago (Sept. 15, 2000)
Published Print	24 years, 11 months ago (Sept. 15, 2000)

Funders 0

None

BibTeX

@article{Angell_2000, title={Relaxation in glassforming liquids and amorphous solids}, volume={88}, ISSN={1089-7550}, url={http://dx.doi.org/10.1063/1.1286035}, DOI={10.1063/1.1286035}, number={6}, journal={Journal of Applied Physics}, publisher={AIP Publishing}, author={Angell, C. A. and Ngai, K. L. and McKenna, G. B. and McMillan, P. F. and Martin, S. W.}, year={2000}, month=sep, pages={3113–3157} }

JSON

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  "publisher": "AIP Publishing",
  "issue": "6",
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  "abstract": "<jats:p>The field of viscous liquid and glassy solid dynamics is reviewed by a process of posing the key questions that need to be answered, and then providing the best answers available to the authors and their advisors at this time. The subject is divided into four parts, three of them dealing with behavior in different domains of temperature with respect to the glass transition temperature, Tg, and a fourth dealing with \u201cshort time processes.\u201d The first part tackles the high temperature regime T&amp;gt;Tg, in which the system is ergodic and the evolution of the viscous liquid toward the condition at Tg is in focus. The second part deals with the regime T\u223cTg, where the system is nonergodic except for very long annealing times, hence has time-dependent properties (aging and annealing). The third part discusses behavior when the system is completely frozen with respect to the primary relaxation process but in which secondary processes, particularly those responsible for \u201csuperionic\u201d conductivity, and dopart mobility in amorphous silicon, remain active. In the fourth part we focus on the behavior of the system at the crossover between the low frequency vibrational components of the molecular motion and its high frequency relaxational components, paying particular attention to very recent developments in the short time dielectric response and the high Q mechanical response.</jats:p>",
  "DOI": "10.1063/1.1286035",
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  "title": "Relaxation in glassforming liquids and amorphous solids",
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