DOI: 10.1063/1.122563. Superradiant lasing from <i>J</i>-aggregated molecules adsorbed onto colloidal silver

Superradiant lasing from J-aggregated molecules adsorbed onto colloidal silver

10.1063/1.122563

Crossref journal-article

AIP Publishing

Applied Physics Letters (317)

Abstract

The picosecond time-resolved emission spectrum of the cyanine dye 1,1′-diethyl-3,3′bis-(3-sulfopropyl)-5,5′,6,6′-tetrachlorobenzimidazolocarbocyanine (also known as BIC) adsorbed onto colloidal silver was examined as a function of laser pulse energy at room temperature. BIC is found to aggregate on colloidal silver, and the number of coherently responding molecules involved in the one-exciton state (i.e., the coherence length) was estimated to involve 8–9 molecules. Lasing at a remarkably low incident pulse energy threshold was found for this system and explained in terms of a mechanism involving superradiant states created in coherently coupled adsorbed molecules that emit photons which stimulate emission from other spatially distributed superradiant states.

Bibliography

ÃzÃ§elik, S., ÃzÃ§elik, I., & Akins, D. L. (1998). Superradiant lasing from J-aggregated molecules adsorbed onto colloidal silver. Applied Physics Letters, 73(14), 1949â1951.

Authors 3

Serdar Özçelik (first)
Isin Özçelik (additional)
Daniel L. Akins (additional)

References 20 Referenced 42

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Dates

Type	When
Created	23 years, 1 month ago (July 26, 2002, 9:31 a.m.)
Deposited	1 year, 6 months ago (Feb. 3, 2024, 10:05 a.m.)
Indexed	1 year, 6 months ago (Feb. 11, 2024, 6:40 a.m.)
Issued	26 years, 10 months ago (Oct. 5, 1998)
Published	26 years, 10 months ago (Oct. 5, 1998)
Published Print	26 years, 10 months ago (Oct. 5, 1998)

Funders 0

None

BibTeX

@article{_z_elik_1998, title={Superradiant lasing from J-aggregated molecules adsorbed onto colloidal silver}, volume={73}, ISSN={1077-3118}, url={http://dx.doi.org/10.1063/1.122563}, DOI={10.1063/1.122563}, number={14}, journal={Applied Physics Letters}, publisher={AIP Publishing}, author={Özçelik, Serdar and Özçelik, Isin and Akins, Daniel L.}, year={1998}, month=oct, pages={1949–1951} }

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