Abstract
We have measured the subpicosecond optical response of a solid-state, semiconductor-to-metal phase transition excited by femtosecond laser pulses. We have determined the dynamic response of the complex refractive index of VO2 thin films by making pump-probe optical transmission and reflection measurements at 780 nm. The phase transition was found to be largely prompt with the optical properties of the high-temperature metallic state being attained within 5 ps. The ultrafast change in complex refractive index enables ultrafast optical switching devices in VO2.
References
13
Referenced
223
{'key': '2024020307502973000_r1'}
10.1126/science.258.5083.770
/ Science (1992){'key': '2024020307502973000_r3'}
10.1016/0038-1098(71)90144-X
/ Solid State Commun. (1971){'key': '2024020307502973000_r5'}
{'key': '2024020307502973000_r6'}
{'key': '2024020307502973000_r7', 'first-page': '430', 'volume': '34', 'year': '1982', 'journal-title': 'JETP Lett.'}
/ JETP Lett. (1982){'key': '2024020307502973000_r8', 'first-page': '887', 'volume': '26', 'year': '1984', 'journal-title': 'Sov. Phys. Solid State'}
/ Sov. Phys. Solid State (1984){'key': '2024020307502973000_r9'}
10.1103/PhysRev.172.788
/ Phys. Rev. (1968)10.1117/12.174076
/ Proc. SPIE (1994)10.1364/OL.16.000324
/ Opt. Lett. (1991)10.1016/0030-4018(85)90120-8
/ Opt. Commun. (1985)
Dates
Type | When |
---|---|
Created | 23 years, 1 month ago (July 26, 2002, 9:38 a.m.) |
Deposited | 1 year, 7 months ago (Feb. 3, 2024, 2:50 a.m.) |
Indexed | 1 month, 1 week ago (July 23, 2025, 8:57 a.m.) |
Issued | 30 years, 11 months ago (Sept. 19, 1994) |
Published | 30 years, 11 months ago (Sept. 19, 1994) |
Published Print | 30 years, 11 months ago (Sept. 19, 1994) |
@article{Becker_1994, title={Femtosecond laser excitation of the semiconductor-metal phase transition in VO2}, volume={65}, ISSN={1077-3118}, url={http://dx.doi.org/10.1063/1.112974}, DOI={10.1063/1.112974}, number={12}, journal={Applied Physics Letters}, publisher={AIP Publishing}, author={Becker, Michael F. and Buckman, A. Bruce and Walser, Rodger M. and Lépine, Thierry and Georges, Patrick and Brun, Alain}, year={1994}, month=sep, pages={1507–1509} }