Direct observation of molecular cooperativity near the glass transition
10.1038/35047037
Crossref journal-article
Springer Science and Business Media LLC
Nature (297)
Authors 2
  1. E. Vidal Russell (first)
  2. N. E. Israeloff (additional)
References 22 Referenced 333
  1. Angell, C. A. Formation of glasses from liquids and biopolymers. Science 267, 1924–1939 (1995). (10.1126/science.267.5206.1924) / Science by CA Angell (1995)
  2. Adam, G. & Gibbs, J. H. On the temperature dependence of cooperative relaxation properties in glass forming liquids. J. Chem. Phys. 43, 139–146 (1965). (10.1063/1.1696442) / J. Chem. Phys. by G Adam (1965)
  3. Weeks, E. R., Crocker, J. L., Levitt, A. C., Schofield, A. & Weitz, D. A. Three-dimensional direct imaging of structural relaxation near the colloidal glass transition. Science 287, 627–629 (2000). (10.1126/science.287.5453.627) / Science by ER Weeks (2000)
  4. Bennemann, C., Donati, C., Baschnagel, J. & Glotzer, S. C. Growing range of correlated motion in a polymer melt on cooling towards the glass transition. Nature 399, 246–249 (1999). (10.1038/20406) / Nature by C Bennemann (1999)
  5. Binder, K., Baschnagel, J., Kob, W. & Paul, W. Glass physics: still not transparent. Phys. World 12, 54 (1999). (10.1088/2058-7058/12/12/16) / Phys. World by K Binder (1999)
  6. Tracht, U. et al. Length scale of dynamic heterogeneities at the glass transition determined by multidimensional nuclear magnetic resonance. Phys. Rev. Lett. 81, 2728–2731 (1998). (10.1103/PhysRevLett.81.2727) / Phys. Rev. Lett. by U Tracht (1998)
  7. Schiener, B., Bohmer, R., Loidl, A. & Chamberlin, R. V. Nonresonant spectral hole burning in the slow dielectric response of supercooled liquids. Science 274, 752–754 (1996). (10.1126/science.274.5288.752) / Science by B Schiener (1996)
  8. Bohmer, R. et al. Nature of the nonexponential primary relaxation in structural glasses probed by dynamically selective experiments. J. Non-Cryst. Solids 235, 1–8 (1998). (10.1016/S0022-3093(98)00581-X) / J. Non-Cryst. Solids by R Bohmer (1998)
  9. Ediger, M. D. Spatially heterogeneous dynamics in supercooled liquids. Annu. Rev. Phys. Chem. 51, (in the press). (10.1146/annurev.physchem.51.1.99)
  10. Dixon, P. K., Wu, L., Nagel, S. R., Williams, B. D. & Carini, J. P. Scaling in the relaxation of a supercooled liquid. Phys. Rev. Lett. 65, 1108–1111 (1990). (10.1103/PhysRevLett.65.1108) / Phys. Rev. Lett. by PK Dixon (1990)
  11. Arbe, A., Colmenero, J., Monkenbusch, M. & Richter, D. Dynamics of glass forming polymers: “homogeneous” vs. “heterogeneous” scenario. Phys. Rev. Lett. 81, 590–593 (1998). (10.1103/PhysRevLett.81.590) / Phys. Rev. Lett. by A Arbe (1998)
  12. Grigera, T. S. & Israeloff, N. E. Observation of fluctuation-dissipation-theorem violations in a structural glass. Phys. Rev. Lett. 83, 5038–5041 (1999). (10.1103/PhysRevLett.83.5038) / Phys. Rev. Lett. by TS Grigera (1999)
  13. Martin, Y., Abraham, D. W. & Wickramasinghe, H. K. High-resolution capacitance measurement and potentiometry by force microscopy. Appl. Phys. Lett. 52, 1103–1105 (1988). (10.1063/1.99224) / Appl. Phys. Lett. by Y Martin (1988)
  14. Walther, L. E., Israeloff, N. E., Vidal Russell, E. & Alvarez Gomariz, H. Mesoscopic scale dielectric relaxation at the glass transition. Phys. Rev. B 57, R15112–R15115 (1998). (10.1103/PhysRevB.57.R15112) / Phys. Rev. B by LE Walther (1998)
  15. Vidal Russell, E., Walther, L. E., Israeloff, N. E. & Alvarez Gomariz, H. Nanometer scale dielectric fluctuations at the glass transition. Phys. Rev. Lett. 81, 1461–1464 (1998). (10.1103/PhysRevLett.81.1461) / Phys. Rev. Lett. by E Vidal Russell (1998)
  16. Walther, L. E., Vidal Russell, E., Israeloff, N. E. & Alvarez Gomariz, H. Atomic force measurement of low frequency dielectric noise. Appl. Phys. Lett. 72, 3223–3226 (1998). (10.1063/1.121556) / Appl. Phys. Lett. by LE Walther (1998)
  17. Albrecht, T. R., Grütter, P., Horne, D. & Rugar, D. Frequency modulation detection using high-Q cantilevers for enhanced force microscope sensitivity. J. Appl. Phys. 69, 668–673 (1991). (10.1063/1.347347) / J. Appl. Phys. by TR Albrecht (1991)
  18. Forrest, J. A., Dalnoki-Veress, K., Stevens, J. R. & Dutcher, J. R. Effect of free surfaces on the glass transition temperature of thin polymer films. Phys. Rev. Lett. 77, 2002–2005 (1996). (10.1103/PhysRevLett.77.2002) / Phys. Rev. Lett. by JA Forrest (1996)
  19. McCrum, N. G., Read, B. E. & Williams, G. Anelastic And Dielectric Effects In Polymeric Solids 302–305 (Dover, New York, 1991). / Anelastic And Dielectric Effects In Polymeric Solids by NG McCrum (1991)
  20. Tracht, U., Heuer, A., Spiess, H. W. Geometry of reorientational dynamics in supercooled poly(vinyl acetate) studied by 2D NMR echo experiments. J. Phys. Chem. 111, 3720–3727 (1999). (10.1063/1.479652) / J. Phys. Chem. by U Tracht (1999)
  21. Xia, X. & Wolynes, P. G. Fragilities of liquids predicted from the random first order transition theory of glasses. Proc. Natl Acad. Sci. USA 97, 2990–2994 (2000). (10.1073/pnas.97.7.2990) / Proc. Natl Acad. Sci. USA by X Xia (2000)
  22. Wang, J. & Wolynes, P. Intermittency of single molecule reaction dynamics in fluctuating environments. Phys. Rev. Lett. 74, 4317–4320 (1995). (10.1103/PhysRevLett.74.4317) / Phys. Rev. Lett. by J Wang (1995)
Dates
Type When
Created 23 years, 1 month ago (July 26, 2002, 4:46 a.m.)
Deposited 2 years, 3 months ago (May 16, 2023, 10:16 p.m.)
Indexed 3 weeks ago (Aug. 6, 2025, 8:58 a.m.)
Issued 24 years, 8 months ago (Dec. 1, 2000)
Published 24 years, 8 months ago (Dec. 1, 2000)
Published Print 24 years, 8 months ago (Dec. 1, 2000)
Funders 0

None

@article{Vidal_Russell_2000, title={Direct observation of molecular cooperativity near the glass transition}, volume={408}, ISSN={1476-4687}, url={http://dx.doi.org/10.1038/35047037}, DOI={10.1038/35047037}, number={6813}, journal={Nature}, publisher={Springer Science and Business Media LLC}, author={Vidal Russell, E. and Israeloff, N. E.}, year={2000}, month=dec, pages={695–698} }