DOI: 10.1021/jp981598o. Assembly and Self-Organization of Silver Nanocrystal Superlattices: Ordered “Soft Spheres”

Assembly and Self-Organization of Silver Nanocrystal Superlattices: Ordered “Soft Spheres”

10.1021/jp981598o

Crossref journal-article

American Chemical Society (ACS)

The Journal of Physical Chemistry B (316)

Bibliography

Korgel, B. A., Fullam, S., Connolly, S., & Fitzmaurice, D. (1998). Assembly and Self-Organization of Silver Nanocrystal Superlattices:â Ordered âSoft Spheres.â The Journal of Physical Chemistry B, 102(43), 8379â8388.

Authors 4

Brian A. Korgel (first)
Stephen Fullam (additional)
Stephen Connolly (additional)
Donald Fitzmaurice (additional)

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For equilibrium to occur at high substrate loadings, the ratio of the particle diffusion and solvent evaporation rates must be close to 1. Assuming steady-state diffusion, the characteristic time, τ, for evaporation of a solvent film of thickness, Δx, is τ = (ρlΔx)/(DsΔc), where ρ is the solvent density (1.483 g/cm3for chloroform); Δcis the concentration gradient in the gas phase (9.4 × 10-4g/cm3for chloroform at 20 °C);Dsis the diffusion coefficient of chloroform vapor in air (∼0.2 cm2/sec); andlis the stagnant diffusion film thickness (∼0.2 μm). When Δx= 200 Å, τ = 0.3 μs for chloroform at 20 °C. The penetration distance (or diffusion length) isx= (4πDpτ)1/2, whereDpis the particle diffusion coefficient. Using the Stokes−Einstein equationDp=kT/6πμRto calculateDp, a 100 Å diameter nanocrystal diffuses 100 Å after τ = 0.3 μs, or one particle diameter. Becausex∝ 1/R1/2,x/Δxis larger for smaller particles, and equilibrium is more easily achieved during solvent evaporation.
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Dates

Type	When
Created	23 years ago (July 26, 2002, 1:28 a.m.)
Deposited	2 years, 4 months ago (March 30, 2023, 9:47 p.m.)
Indexed	4 hours, 57 minutes ago (Aug. 23, 2025, 12:58 a.m.)
Issued	26 years, 10 months ago (Oct. 1, 1998)
Published	26 years, 10 months ago (Oct. 1, 1998)
Published Online	26 years, 10 months ago (Oct. 1, 1998)
Published Print	26 years, 10 months ago (Oct. 1, 1998)

Funders 0

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BibTeX

@article{Korgel_1998, title={Assembly and Self-Organization of Silver Nanocrystal Superlattices: Ordered “Soft Spheres”}, volume={102}, ISSN={1520-5207}, url={http://dx.doi.org/10.1021/jp981598o}, DOI={10.1021/jp981598o}, number={43}, journal={The Journal of Physical Chemistry B}, publisher={American Chemical Society (ACS)}, author={Korgel, Brian A. and Fullam, Stephen and Connolly, Stephen and Fitzmaurice, Donald}, year={1998}, month=oct, pages={8379–8388} }

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