DOI: 10.1021/jp021494k. Ionic and Neutral Species in Pulse Radiolysis of Supercritical CO<sub>2</sub>. 1. Transient Absorption Spectroscopy, Electric Field Effect, and Charge Dynamics

Ionic and Neutral Species in Pulse Radiolysis of Supercritical CO2. 1. Transient Absorption Spectroscopy, Electric Field Effect, and Charge Dynamics

10.1021/jp021494k

Crossref journal-article

American Chemical Society (ACS)

The Journal of Physical Chemistry A (316)

Bibliography

Shkrob, I. A., Sauer, M. C., Jonah, C. D., & Takahashi, K. (2002). Ionic and Neutral Species in Pulse Radiolysis of Supercritical CO2. 1. Transient Absorption Spectroscopy, Electric Field Effect, and Charge Dynamics. The Journal of Physical Chemistry A, 106(49), 11855â11870.

Authors 4

Ilya A. Shkrob (first)
Myran C. Sauer (additional)
Charles D. Jonah (additional)
Kenji Takahashi (additional)

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In this optical time-of-flight experiment, the loss of the ions because of their discharge at the electrodes is observed. Under our experimental conditions, the drift of the ions is stalled by the space charge in the sample (see ref 21). Assuming that the ions do not recombine, we found, by numerical simulations, that for an initial ion concentration of 1 μM and a field of 25 kV/cm ca. 20% of the ions will be neutralized at the electrodes att= 5 ms (for typical ion mobilities of μ+= 2 × 10-3cm2/Vs and μ-= 4 × 10-3cm2/Vs, ref 4). For an initial concentration of 100 nM, the same fraction of ions will be neutralized at 2 ms; the lower the concentration, the faster the ion decay. Because we have not observed any field-induced loss of the 550 nm absorbance on the 1−100 ms time scale, the conclusion is that the product is not an (unusually stable) ion.
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Dates

Type	When
Created	22 years, 8 months ago (Dec. 5, 2002, 12:34 a.m.)
Deposited	2 years, 4 months ago (April 2, 2023, 12:13 p.m.)
Indexed	2 years ago (Aug. 4, 2023, 1:33 a.m.)
Issued	22 years, 9 months ago (Nov. 7, 2002)
Published	22 years, 9 months ago (Nov. 7, 2002)
Published Online	22 years, 9 months ago (Nov. 7, 2002)
Published Print	22 years, 8 months ago (Dec. 1, 2002)

Funders 0

None

BibTeX

@article{Shkrob_2002, title={Ionic and Neutral Species in Pulse Radiolysis of Supercritical CO2. 1. Transient Absorption Spectroscopy, Electric Field Effect, and Charge Dynamics}, volume={106}, ISSN={1520-5215}, url={http://dx.doi.org/10.1021/jp021494k}, DOI={10.1021/jp021494k}, number={49}, journal={The Journal of Physical Chemistry A}, publisher={American Chemical Society (ACS)}, author={Shkrob, Ilya A. and Sauer, Myran C. and Jonah, Charles D. and Takahashi, Kenji}, year={2002}, month=nov, pages={11855–11870} }

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