DOI: 10.1002/ange.201712952. Nanoskalige chemische Bildgebung von Zeolithen durch Atomsondentomographie

Nanoskalige chemische Bildgebung von Zeolithen durch Atomsondentomographie

10.1002/ange.201712952

Crossref journal-article

Wiley

Angewandte Chemie (311)

Abstract

AbstractStruktur‐Zusammensetzungs‐Eigenschafts‐Beziehungen für zeolithbasierte Materialien sind entscheidend, um verbesserte Feststoffkatalysatoren zu entwickeln. Die Realisierung kann sich jedoch als schwierig erweisen, da sogar einzelne Zeolithkristalle Heterogenitäten aufweisen können, die sich auf Reaktivität, Diffusion und Stabilität auswirken können. Mithilfe von tomographischen Verfahren wurden Fortschritte bei der Charakterisierung dieser porösen Feststoffe erreicht, allerdings haben alle Methoden eine begrenzte räumliche Auflösung. Nur die Atomsondentomographie (APT) ist bisher in der Lage, 3D‐Rekonstruktionen mit Subnanometer‐Auflösung zu erzeugen. Hier behandeln wir die Untersuchung von Zeolithen mit APT: Hierzu gehören Aspekte der Probenvorbereitung, die Datenerfassung, die Signalzuordnung in Massenspektren, die kristallographische Auflösungsgrenze und eine genaue Datenanalyse. Sämtliche Abschnitte werden mit Beispielen erläutert. Zudem sollen bisher unveröffentlichte Daten und Analysen praktische Strategien aufzeigen, die mögliche Probleme des Einsatzes der APT bei Zeolithen lösen.

Bibliography

Schmidt, J. E., Peng, L., Poplawsky, J. D., & Weckhuysen, B. M. (2018). Nanoskalige chemische Bildgebung von Zeolithen durch Atomsondentomographie. Angewandte Chemie, 130(33), 10580â10593. Portico.

Authors 4

Joel E. Schmidt (first)
Linqing Peng (additional)
Jonathan D. Poplawsky (additional)
Bert M. Weckhuysen (additional)

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Dates

Type	When
Created	7 years, 3 months ago (May 2, 2018, 9:12 a.m.)
Deposited	1 year, 11 months ago (Sept. 10, 2023, 8:04 p.m.)
Indexed	6 months ago (Feb. 20, 2025, 9:19 p.m.)
Issued	7 years, 1 month ago (July 24, 2018)
Published	7 years, 1 month ago (July 24, 2018)
Published Online	7 years, 1 month ago (July 24, 2018)
Published Print	7 years ago (Aug. 13, 2018)

Funders 3

H2020 European Research Council 10.13039/100010663
Region: Europe
gov (National government)
Labels17
1. H2020 Excellent Science - European Research Council
2. European Research Council
3. H2020 Wissenschaftsexzellenz - Für das Einzelziel 'Europäischer Forschungsrat (ERC)'
4. H2020 Ciencia Excelente - Consejo Europeo de Investigación (CEI)
5. H2020 Excellence Scientifique - Conseil européen de la recherche (CER)
6. H2020 Eccellenza Scientifica - Consiglio europeo della ricerca (CER)
7. H2020 Doskonała Baza Naukowa - Europejska Rada ds. Badań Naukowych (ERBN)
8. EXCELLENT SCIENCE - European Research Council
9. WISSENSCHAFTSEXZELLENZ - Für das Einzelziel 'Europäischer Forschungsrat
10. CIENCIA EXCELENTE - Consejo Europeo de Investigación
11. EXCELLENCE SCIENTIFIQUE - Conseil européen de la recherche
12. ECCELLENZA SCIENTIFICA - Consiglio europeo della ricerca
13. DOSKONAŁA BAZA NAUKOWA - Europejska Rada ds. Badań Naukowych
14. ERC
15. CEI
16. CER
17. ERBN
Awards1
1. Advanced Research Grant (no.321140)
Nederlandse Organisatie voor Wetenschappelijk Onderzoek 10.13039/501100003246
Region: Europe
gov (National government)
Labels9
1. Netherlands Organisation for Scientific Research
2. Dutch National Scientific Foundation
3. Dutch National Science Foundation
4. Dutch Research Council (Nederlandse Organisatie voor Wetenschappelijk Onderzoek)
5. NWO:Nederlandse Organisatie voor Wetenschappelijk Onderzoek
6. Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO)
7. Dutch Research Council
8. Dutch Research Council, Netherlands
9. NWO
Awards1
1. Gravitation Program - Multiscale Catalytic Energy Conversion (MCEC)
Horizon 2020 Framework Programme 10.13039/100010661
Region: Europe
gov (National government)
Labels13
1. EU Framework Programme for Research and Innovation H2020
2. Horizon 2020
3. Rahmenprogramm Horizont 2020
4. Programa Marco Horizonte 2020
5. Programme-cadre Horizon 2020
6. Programma quadro Orizzonte 2020
7. Program ramowy Horyzont 2020
8. Horizont 2020
9. Horizonte 2020
10. Orizzonte 2020
11. Horyzont 2020
12. Horizon 2020 Framework Programme (H2020)
13. H2020
Awards1
1. Marie Sklodowska-Curie grant agreement No. 702149

BibTeX

@article{Schmidt_2018, title={Nanoskalige chemische Bildgebung von Zeolithen durch Atomsondentomographie}, volume={130}, ISSN={1521-3757}, url={http://dx.doi.org/10.1002/ange.201712952}, DOI={10.1002/ange.201712952}, number={33}, journal={Angewandte Chemie}, publisher={Wiley}, author={Schmidt, Joel E. and Peng, Linqing and Poplawsky, Jonathan D. and Weckhuysen, Bert M.}, year={2018}, month=jul, pages={10580–10593} }

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