DOI: 10.1002/adma.201700008. Tri‐<i>s</i>‐triazine‐Based Crystalline Carbon Nitride Nanosheets for an Improved Hydrogen Evolution

Tri‐s‐triazine‐Based Crystalline Carbon Nitride Nanosheets for an Improved Hydrogen Evolution

10.1002/adma.201700008

Crossref journal-article

Wiley

Advanced Materials (311)

Abstract

Tri‐s‐triazine‐based crystalline carbon nitride nanosheets (CCNNSs) have been successfully extracted via a conventional and cost‐effective sonication–centrifugation process. These CCNNSs possess a highly defined and unambiguous structure with minimal thickness, large aspect ratios, homogeneous tri‐s‐triazine‐based units, and high crystallinity. These tri‐s‐triazine‐based CCNNSs show significantly enhanced photocatalytic hydrogen generation activity under visible light than g‐C3N4, poly (triazine imide)/Li+ Cl–, and bulk tri‐s‐triazine‐based crystalline carbon nitrides. A highly apparent quantum efficiency of 8.57% at 420 nm for hydrogen production from aqueous methanol feedstock can be achieved from tri‐s‐triazine‐based CCNNSs, exceeding most of the reported carbon nitride nanosheets. Benefiting from the inherent structure of 2D crystals, the ultrathin tri‐s‐triazine‐based CCNNSs provide a broad range of application prospects in the fields of bioimaging, and energy storage and conversion.

Bibliography

Ou, H., Lin, L., Zheng, Y., Yang, P., Fang, Y., & Wang, X. (2017). TriâsâtriazineâBased Crystalline Carbon Nitride Nanosheets for an Improved Hydrogen Evolution. Advanced Materials, 29(22). Portico.

Authors 6

Honghui Ou (first)
Lihua Lin (additional)
Yun Zheng (additional)
Pengju Yang (additional)
Yuanxing Fang (additional)
Xinchen Wang (additional)

References 50 Referenced 618

Dates

Type	When
Created	8 years, 4 months ago (April 12, 2017, 2:02 a.m.)
Deposited	1 year, 11 months ago (Sept. 15, 2023, 10:43 p.m.)
Indexed	57 minutes ago (Aug. 29, 2025, 5:43 a.m.)
Issued	8 years, 4 months ago (April 12, 2017)
Published	8 years, 4 months ago (April 12, 2017)
Published Online	8 years, 4 months ago (April 12, 2017)
Published Print	8 years, 2 months ago (June 1, 2017)

Funders 1

National Natural Science Foundation of China 10.13039/501100001809
Region: Asia
gov (National government)
Labels11
1. Chinese National Science Foundation
2. Natural Science Foundation of China
3. National Science Foundation of China
4. NNSF of China
5. NSF of China
6. 国家自然科学基金委员会
7. National Nature Science Foundation of China
8. Guójiā Zìrán Kēxué Jījīn Wěiyuánhuì
9. NSFC
10. NNSF
11. NNSFC
Awards2
1. 2161101090
2. 21425309

BibTeX

@article{Ou_2017, title={Tri‐s‐triazine‐Based Crystalline Carbon Nitride Nanosheets for an Improved Hydrogen Evolution}, volume={29}, ISSN={1521-4095}, url={http://dx.doi.org/10.1002/adma.201700008}, DOI={10.1002/adma.201700008}, number={22}, journal={Advanced Materials}, publisher={Wiley}, author={Ou, Honghui and Lin, Lihua and Zheng, Yun and Yang, Pengju and Fang, Yuanxing and Wang, Xinchen}, year={2017}, month=apr }

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